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Atomistic Simulation of HF Etching Process of Amorphous $\mathrm{Si}_3\mathrm{N}_4$ Using Machine Learning Potential
Changho Hong, $^{\parallel}$ Sangmin Oh, $^{\parallel}$ Hyungmin An, Purun-hanul Kim, Yaeji Kim, Jae-hyeon Ko, Jiwoong Sue, Dongyean Oh, Sungkye Park, and Seungwu Han*
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Plasma etching
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Atomistic Simulation of HF Etching Process of Amorphous $\mathrm{Si}_3\mathrm{N}_4$ Using Machine Learning Potential
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Figure 1. Schematic of the data set construction for NNP training. Initial baseline structures cover diverse equilibrium configurations. Reaction-specific sets are captured via guided MD, while general-purpose sets are derived from high-temperature MD simulations. Iterative refinements of the NNP are conducted using tr...
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Atomistic Simulation of HF Etching Process of Amorphous $\mathrm{Si}_3\mathrm{N}_4$ Using Machine Learning Potential
Changho Hong, $^{\parallel}$ Sangmin Oh, $^{\parallel}$ Hyungmin An, Purun-hanul Kim, Yaeji Kim, Jae-hyeon Ko, Jiwoong Sue, Dongyean Oh, Sungkye Park, and Seungwu Han*
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Figure 10. Number distribution of etching products with regard to $\theta_{\mathrm{in}}$ . The error bars indicate the standard deviations among three independent runs.
sci_imageminer__atomic_layer_etching__simulation_usecase__33__figure_10
atomic-layer-etching/simulation-usecase/33/figure_10
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[ { "panel_id": "a", "summary": "The grouped bar chart displays the number of molecular products generated for a range of gas species—including SiFₓ (x = 1–4), N-based species (N, NH, NH₂, NH₃, N₂), and composite species (SiₓNᵧ)—as a function of incident angle from 0° to 75°. Fluorinated silicon products like...
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Atomistic Simulation of HF Etching Process of Amorphous $\mathrm{Si}_3\mathrm{N}_4$ Using Machine Learning Potential
Changho Hong, $^{\parallel}$ Sangmin Oh, $^{\parallel}$ Hyungmin An, Purun-hanul Kim, Yaeji Kim, Jae-hyeon Ko, Jiwoong Sue, Dongyean Oh, Sungkye Park, and Seungwu Han*
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Figure 11. Schematic of atomistic mechanism in $\mathrm{Si}_3\mathrm{N}_4$ etching (a) at low angle of incidence, and (b) high angle of incidence.
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Atomistic Simulation of HF Etching Process of Amorphous $\mathrm{Si}_3\mathrm{N}_4$ Using Machine Learning Potential
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Figure 12. Evolution of populations of surface species $(N_{i})$ in the modified layer as a function of HF dose. The solid lines are the results of 1D continuum model while symbols are directly obtained from MD simulations with $E_{\mathrm{in}}$ of $50~\mathrm{eV}$ and $\theta_{\mathrm{in}}$ of $0^{\circ}$ . P...
sci_imageminer__atomic_layer_etching__simulation_usecase__33__figure_12
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[ { "panel_id": "a", "data": "| Dose (HF/nm²) | N (nm⁻²) | NH₀ (nm⁻²) | NH₁ (nm⁻²) | NH₂ (nm⁻²) |\n|---------------|-----------|-------------|-------------|-------------|\n| 0 | 35 | 10 | 0 | 0 |\n| 50 | 30 | 8 | 5 | 2 ...
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Atomistic Simulation of HF Etching Process of Amorphous $\mathrm{Si}_3\mathrm{N}_4$ Using Machine Learning Potential
Changho Hong, $^{\parallel}$ Sangmin Oh, $^{\parallel}$ Hyungmin An, Purun-hanul Kim, Yaeji Kim, Jae-hyeon Ko, Jiwoong Sue, Dongyean Oh, Sungkye Park, and Seungwu Han*
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Figure 3. (a) Comparison of the DFT and NNP energies along the NNP MD trajectory for the crystalline slab after the primitive training and (b) the etched surface after the NNP MD simulation. (b)
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Atomistic Simulation of HF Etching Process of Amorphous $\mathrm{Si}_3\mathrm{N}_4$ Using Machine Learning Potential
Changho Hong, $^{\parallel}$ Sangmin Oh, $^{\parallel}$ Hyungmin An, Purun-hanul Kim, Yaeji Kim, Jae-hyeon Ko, Jiwoong Sue, Dongyean Oh, Sungkye Park, and Seungwu Han*
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Figure 4. Comparison of reaction energies during etching MD calculated using DFT $(E_{\mathrm{rxn}}^{\mathrm{DFT}})$ and NNP $(E_{\mathrm{rxn}}^{\mathrm{NNP}})$ . Each point refers to individual reactions. The density of data points on the color bar indicates the local density of reaction events in the vicinity of e...
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Atomistic Simulation of HF Etching Process of Amorphous $\mathrm{Si}_3\mathrm{N}_4$ Using Machine Learning Potential
Changho Hong, $^{\parallel}$ Sangmin Oh, $^{\parallel}$ Hyungmin An, Purun-hanul Kim, Yaeji Kim, Jae-hyeon Ko, Jiwoong Sue, Dongyean Oh, Sungkye Park, and Seungwu Han*
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(a) Figure 6. (a) The number of Si, N, H, and F atoms in the simulation cell during the etching process at $E_{\mathrm{in}} = 50 \mathrm{eV}$ and $\theta_{\mathrm{in}} = 0^{\circ}$ . (b) Etching yield as a function of incident energy. The black dashed line represents the fitted function of the universal etching beha...
sci_imageminer__atomic_layer_etching__simulation_usecase__33__figure_6
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[ { "panel_id": "a", "summary": "This figure presents the number of Si, N, H, and F atoms in a system as a function of HF dose. As HF exposure increases from 0 to 200 HF/nm², both silicon (Si) and nitrogen (N) atoms show a steady decline, indicating progressive etching or transformation. Fluorine (F) atoms in...
[ { "panel_id": "a", "data": "| Dose (HF/nm²) | Si | N | H | F |\n|---------------|----|----|----|----|\n| 0 | 400 | 500 | 100 | 0 |\n| 50 | 370 | 460 | 110 | 120 |\n| 100 | 340 | 420 | 110 | 140 |\n| 150 | 310 | 390 | 110 | 150 |\n| 200 | 280 | 360 | 110...
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Atomistic Simulation of HF Etching Process of Amorphous $\mathrm{Si}_3\mathrm{N}_4$ Using Machine Learning Potential
Changho Hong, $^{\parallel}$ Sangmin Oh, $^{\parallel}$ Hyungmin An, Purun-hanul Kim, Yaeji Kim, Jae-hyeon Ko, Jiwoong Sue, Dongyean Oh, Sungkye Park, and Seungwu Han*
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Atomistic Simulation of HF Etching Process of Amorphous.pdf
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Figure 7. Number distribution of etching products with regard to $E_{\mathrm{in}}$ . The error bars indicate the standard deviations among three independent runs.
sci_imageminer__atomic_layer_etching__simulation_usecase__33__figure_7
atomic-layer-etching/simulation-usecase/33/figure_7
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[ { "panel_id": "a", "label": "grouped bar chart" } ]
[ { "panel_id": "a", "summary": "This grouped bar chart illustrates how the formation of various gas-phase species evolves with increasing incident energy from 10 eV to 50 eV. Fluorinated silicon products (e.g., SiF₂, SiF₃, SiF₄) show a marked increase with energy, with SiF₄ becoming the dominant species at e...
[ { "panel_id": "a", "data": "| Gas species | Si | SiF | SiF₂ | SiF₃ | SiF₄ | N | NH | NH₂ | NH₃ | N₂ | SiₓNy |\n|---|---|---|---|---|---|---|---|---|---|---|---|\n| 10 eV | 0 | 0 | 0 | 0 | 0 | 0 | 0 | 0 | 15 | 5 | 0 |\n| 20 eV | 0 | 0 | 0 | 0 | 5 | 0 | 0 | 0 | 30 | 10 | 0 |\n| 30 eV | 0 | 0 | 5 | 5 | 35 | 0 ...
[ { "panel_id": "a", "question_type": "Structure-Property", "question": "How does increasing the incident energy affect the distribution of gas species observed in the reaction?", "answer_type": "Paragraph", "answer": "As the incident energy increases from 10 eV to 50 eV, the number of fluorinated...
[ { "panel_id": "a", "x": 0, "y": 0, "width": 875, "height": 414 } ]
{ "publication_title": "Atomistic Simulation of HF Etching Process of Amorphous $\\mathrm{Si}_3\\mathrm{N}_4$ Using Machine Learning Potential", "authors": "Changho Hong, $^{\\parallel}$ Sangmin Oh, $^{\\parallel}$ Hyungmin An, Purun-hanul Kim, Yaeji Kim, Jae-hyeon Ko, Jiwoong Sue, Dongyean Oh, Sungkye Park, an...
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Atomistic Simulation of HF Etching Process of Amorphous $\mathrm{Si}_3\mathrm{N}_4$ Using Machine Learning Potential
Changho Hong, $^{\parallel}$ Sangmin Oh, $^{\parallel}$ Hyungmin An, Purun-hanul Kim, Yaeji Kim, Jae-hyeon Ko, Jiwoong Sue, Dongyean Oh, Sungkye Park, and Seungwu Han*
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Atomistic Simulation of HF Etching Process of Amorphous.pdf
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Figure 8. (a–f) The etched surfaces of $\mathrm{a - Si_3N_4}$ with regard to the angle of incidence $(\theta_{\mathrm{in}})$ of HF: $\theta_{\mathrm{in}} = 0, 15, 30, 45, 60$ and $75^{\circ}$ , respectively. The kinetic energy of the HF molecule is $50~\mathrm{eV}$ . The initial height of the surface before etc...
sci_imageminer__atomic_layer_etching__simulation_usecase__33__figure_8
atomic-layer-etching/simulation-usecase/33/figure_8
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[ { "panel_id": "a", "label": "molecular structure diagram" } ]
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{ "publication_title": "Atomistic Simulation of HF Etching Process of Amorphous $\\mathrm{Si}_3\\mathrm{N}_4$ Using Machine Learning Potential", "authors": "Changho Hong, $^{\\parallel}$ Sangmin Oh, $^{\\parallel}$ Hyungmin An, Purun-hanul Kim, Yaeji Kim, Jae-hyeon Ko, Jiwoong Sue, Dongyean Oh, Sungkye Park, an...
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Atomistic Simulation of HF Etching Process of Amorphous $\mathrm{Si}_3\mathrm{N}_4$ Using Machine Learning Potential
Changho Hong, $^{\parallel}$ Sangmin Oh, $^{\parallel}$ Hyungmin An, Purun-hanul Kim, Yaeji Kim, Jae-hyeon Ko, Jiwoong Sue, Dongyean Oh, Sungkye Park, and Seungwu Han*
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Figure 9. (a) The reflection coefficient, and (b) the total etching yield per incident HF molecule, both as a function of the incident angle. The error bars indicate the standard deviations among three independent runs.
sci_imageminer__atomic_layer_etching__simulation_usecase__33__figure_9
atomic-layer-etching/simulation-usecase/33/figure_9
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[ { "panel_id": "a", "label": "line chart" } ]
[ { "panel_id": "a", "summary": "The figure presents the variation of reflection coefficient as a function of incident angle (θ<sub>in</sub>) from 0° to 75°. From 0° to 45°, the reflection coefficient remains relatively constant at around 0.1, indicating minimal reflection changes over low to moderate angles....
[ { "panel_id": "a", "data": "| θ<sub>in</sub> (deg) | Reflection coefficient |\n|---|---|\n| 0 | 0.1 |\n| 15 | 0.1 |\n| 30 | 0.1 |\n| 45 | 0.1 |\n| 60 | 0.2 |\n| 75 | 0.45 |" } ]
[ { "panel_id": "a", "question_type": "Structure-Property", "question": "How does the reflection coefficient respond to changes in the incident angle θ<sub>in</sub>?", "answer_type": "Paragraph", "answer": "The reflection coefficient remains relatively stable at around 0.1 between 0° and 45°, sugg...
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{ "publication_title": "Atomistic Simulation of HF Etching Process of Amorphous $\\mathrm{Si}_3\\mathrm{N}_4$ Using Machine Learning Potential", "authors": "Changho Hong, $^{\\parallel}$ Sangmin Oh, $^{\\parallel}$ Hyungmin An, Purun-hanul Kim, Yaeji Kim, Jae-hyeon Ko, Jiwoong Sue, Dongyean Oh, Sungkye Park, an...
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Atomistic Simulation of HF Etching Process of Amorphous $\mathrm{Si}_3\mathrm{N}_4$ Using Machine Learning Potential
Changho Hong, $^{\parallel}$ Sangmin Oh, $^{\parallel}$ Hyungmin An, Purun-hanul Kim, Yaeji Kim, Jae-hyeon Ko, Jiwoong Sue, Dongyean Oh, Sungkye Park, and Seungwu Han*
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Atomistic Simulation of HF Etching Process of Amorphous.pdf
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sci_imageminer__atomic_layer_etching__simulation_usecase__35__435b0c42ea89c8d2de2dcaea88e499aa20a402f2b076777162ac90d4a10d1a1c
atomic-layer-etching/simulation-usecase/35/435b0c42ea89c8d2de2dcaea88e499aa20a402f2b076777162ac90d4a10d1a1c
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[ { "panel_id": "a", "label": "molecular structure diagram" }, { "panel_id": "b", "label": "scatter plot" } ]
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{ "publication_title": "Density Functional Theory Study of Oxygen Adsorption on Polymer Surfaces for Atomic-Layer Etching: Implications for Semiconductor Device Fabrication", "authors": "Roberto C. Longo, Alok Ranjan, and Peter L. G. Ventzek*", "doi": null, "doi_candidates": [ "10.1021/acsanm.0c00618" ], ...
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Density Functional Theory Study of Oxygen Adsorption on Polymer Surfaces for Atomic-Layer Etching: Implications for Semiconductor Device Fabrication
Roberto C. Longo, Alok Ranjan, and Peter L. G. Ventzek*
null
null
2,020
Density Functional Theory Study of Oxygen Adsorption on Polymer Surfaces for Atomic-Layer.pdf
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Figure 1. Schematic representation of the use of organic masks in ideal ALE (a) and ALD (b) cycles.
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[ { "panel_id": "a", "label": "process flow diagram" } ]
[ { "panel_id": "a", "summary": "The figure shows a plasma-based surface processing sequence on a wafer. First, plasma species interact with an organic layer on the substrate. After this step, parts of the organic layer remain and act as a mask. The figure illustrates how plasma exposure leads to mask formati...
[ { "panel_id": "a", "data": "" } ]
[ { "panel_id": "a", "question_type": "Process-Oriented", "question": "What is the role of the plasma during the initial stage shown in the figure?", "answer_type": "Paragraph", "answer": "The plasma supplies reactive species that interact with the organic surface layer. These species modify the c...
[ { "panel_id": "a", "x": 3, "y": 0, "width": 1032, "height": 297 } ]
{ "publication_title": "Density Functional Theory Study of Oxygen Adsorption on Polymer Surfaces for Atomic-Layer Etching: Implications for Semiconductor Device Fabrication", "authors": "Roberto C. Longo, Alok Ranjan, and Peter L. G. Ventzek*", "doi": null, "doi_candidates": [ "10.1021/acsanm.0c00618" ], ...
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Density Functional Theory Study of Oxygen Adsorption on Polymer Surfaces for Atomic-Layer Etching: Implications for Semiconductor Device Fabrication
Roberto C. Longo, Alok Ranjan, and Peter L. G. Ventzek*
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Density Functional Theory Study of Oxygen Adsorption on Polymer Surfaces for Atomic-Layer.pdf
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(a)
sci_imageminer__atomic_layer_etching__simulation_usecase__35__fig1_a
atomic-layer-etching/simulation-usecase/35/FIG1_a
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[ { "panel_id": "a", "label": "process flow diagram" } ]
[ { "panel_id": "a", "summary": "The first step shows precursor-1 exposure to the masked surface, where the precursor selectively interacts with the exposed regions to form a modified surface layer. This step defines the spatial selectivity of the process and prepares the surface chemistry for the subsequent ...
[ { "panel_id": "a", "data": "" } ]
[ { "panel_id": "a", "question_type": "Process-Oriented", "question": "Why are purge steps inserted between the precursor exposure and plasma stages?", "answer_type": "Paragraph", "answer": "The purge steps remove unreacted precursor molecules and gaseous by-products from the chamber. This prevent...
[ { "panel_id": "a", "x": 4, "y": 6, "width": 673, "height": 334 } ]
{ "publication_title": "Density Functional Theory Study of Oxygen Adsorption on Polymer Surfaces for Atomic-Layer Etching: Implications for Semiconductor Device Fabrication", "authors": "Roberto C. Longo, Alok Ranjan, and Peter L. G. Ventzek*", "doi": null, "doi_candidates": [ "10.1021/acsanm.0c00618" ], ...
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Density Functional Theory Study of Oxygen Adsorption on Polymer Surfaces for Atomic-Layer Etching: Implications for Semiconductor Device Fabrication
Roberto C. Longo, Alok Ranjan, and Peter L. G. Ventzek*
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Density Functional Theory Study of Oxygen Adsorption on Polymer Surfaces for Atomic-Layer.pdf
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sci_imageminer__atomic_layer_etching__simulation_usecase__35__fig1_b
atomic-layer-etching/simulation-usecase/35/FIG1_b
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[ { "panel_id": "a", "label": "process flow diagram" } ]
[ { "panel_id": "a", "summary": "The figure shows a stepwise surface deposition process using two different precursors. In the first step, precursor-1 reacts only with exposed surface regions, forming a fraction of a monolayer. After a purge, precursor-2 reacts with the remaining sites to complete the monolay...
[ { "panel_id": "a", "data": "" } ]
[ { "panel_id": "a", "question_type": "Process-Oriented", "question": "Why does the first precursor step result in only a fraction of a monolayer rather than full coverage?", "answer_type": "Paragraph", "answer": "During the first step, only surface regions that are not protected by the mask are a...
[ { "panel_id": "a", "x": 2, "y": 4, "width": 711, "height": 370 } ]
{ "publication_title": "Density Functional Theory Study of Oxygen Adsorption on Polymer Surfaces for Atomic-Layer Etching: Implications for Semiconductor Device Fabrication", "authors": "Roberto C. Longo, Alok Ranjan, and Peter L. G. Ventzek*", "doi": null, "doi_candidates": [ "10.1021/acsanm.0c00618" ], ...
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Density Functional Theory Study of Oxygen Adsorption on Polymer Surfaces for Atomic-Layer Etching: Implications for Semiconductor Device Fabrication
Roberto C. Longo, Alok Ranjan, and Peter L. G. Ventzek*
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Density Functional Theory Study of Oxygen Adsorption on Polymer Surfaces for Atomic-Layer.pdf
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Figure 2. Lateral and front views of the PS surface model used in the calculations. Brown spheres represent carbon atoms, and white spheres represent hydrogen atoms.
sci_imageminer__atomic_layer_etching__simulation_usecase__35__fig2
atomic-layer-etching/simulation-usecase/35/FIG2
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[ { "panel_id": "a", "label": "molecular structure diagram" }, { "panel_id": "b", "label": "molecular structure diagram" }, { "panel_id": "c", "label": "molecular structure diagram" } ]
[ { "panel_id": "a", "summary": "This panel shows a dense, three-dimensional molecular model of bulk polystyrene. Many polymer chains are packed together, forming an entangled network. Individual chains are hard to distinguish at this scale." }, { "panel_id": "b", "summary": "A local segment of th...
[ { "panel_id": "a", "data": "" }, { "panel_id": "b", "data": "" }, { "panel_id": "c", "data": "" } ]
[ { "panel_id": "a", "question_type": "Process-Oriented", "question": "Why is a local segment extracted from the bulk polystyrene structure?", "answer_type": "Paragraph", "answer": "The bulk structure is very dense and visually complex. Extracting a local segment removes interference from neighbor...
[ { "panel_id": "a", "x": 1, "y": 5, "width": 549, "height": 517 }, { "panel_id": "b", "x": 1, "y": 5, "width": 549, "height": 517 }, { "panel_id": "c", "x": 496, "y": 270, "width": 385, "height": 248 } ]
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Density Functional Theory Study of Oxygen Adsorption on Polymer Surfaces for Atomic-Layer Etching: Implications for Semiconductor Device Fabrication
Roberto C. Longo, Alok Ranjan, and Peter L. G. Ventzek*
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Density Functional Theory Study of Oxygen Adsorption on Polymer Surfaces for Atomic-Layer.pdf
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sci_imageminer__atomic_layer_etching__simulation_usecase__35__fig3
atomic-layer-etching/simulation-usecase/35/FIG3
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[ { "panel_id": "a", "label": "molecular structure diagram" }, { "panel_id": "b", "label": "molecular structure diagram" }, { "panel_id": "c", "label": "molecular structure diagram" }, { "panel_id": "d", "label": "molecular structure diagram" }, { "panel_id": "e", ...
[ { "panel_id": "a", "summary": "The structure shows the intact molecular backbone with a single oxygen added at an isolated site. The overall geometry remains unchanged." }, { "panel_id": "b", "summary": "A second oxygen binds near the first site, causing a small local rearrangement but no global...
[ { "panel_id": "a", "data": "" }, { "panel_id": "b", "data": "" }, { "panel_id": "c", "data": "" }, { "panel_id": "d", "data": "" }, { "panel_id": "e", "data": "" }, { "panel_id": "f", "data": "" }, { "panel_id": "g", "data": "" }, {...
[ { "panel_id": "j", "question_type": "Comparative/Trend", "question": "What is the most direct trend when comparing O₆ to O₁₀?", "answer_type": "Factoid", "answer": "Oxygen incorporation increases from six to ten." }, { "panel_id": "k", "question_type": "Structure-Property", "ques...
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{ "publication_title": "Density Functional Theory Study of Oxygen Adsorption on Polymer Surfaces for Atomic-Layer Etching: Implications for Semiconductor Device Fabrication", "authors": "Roberto C. Longo, Alok Ranjan, and Peter L. G. Ventzek*", "doi": null, "doi_candidates": [ "10.1021/acsanm.0c00618" ], ...
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Density Functional Theory Study of Oxygen Adsorption on Polymer Surfaces for Atomic-Layer Etching: Implications for Semiconductor Device Fabrication
Roberto C. Longo, Alok Ranjan, and Peter L. G. Ventzek*
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2,020
Density Functional Theory Study of Oxygen Adsorption on Polymer Surfaces for Atomic-Layer.pdf
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Figure 4. Scatter plot showing the adsorption energy versus oxygen coverage of the minima shown in Figure 3. All of the points were fit to a parabola for eye-guiding purposes. The highlighted points are cross-referenced to the configurations shown in Figure 3. Brown, white, and red spheres represent carbon, hydrogen, a...
sci_imageminer__atomic_layer_etching__simulation_usecase__35__fig4
atomic-layer-etching/simulation-usecase/35/FIG4
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[ { "panel_id": "a", "label": "scatter plot" } ]
[ { "panel_id": "a", "summary": "The figure shows adsorption energy as oxygen coverage increases. At low coverage, adsorption is strongly favorable. Stable species such as H₂O are formed. At higher coverage, adsorption becomes less stable. New bonds form and the polymer structure begins to break." } ]
[ { "panel_id": "a", "data": "| Coverage [O/nm²] | Adsorption Energy [eV/nm²] | Annotated chemical event |\n|------------------|----------------------------|--------------------------|\n| 0.5 | −2.02 (global minimum) | Initial adsorption |\n| 3.0 | −1.00 (local minimum) | H₂...
[ { "panel_id": "a", "question_type": "Process-Oriented", "question": "How does increasing oxygen coverage change the dominant surface reactions observed on polystyrene?", "answer_type": "Paragraph", "answer": "At low oxygen coverage, reactions favor stable adsorption and low-energy products such ...
[ { "panel_id": "a", "x": 3, "y": 2, "width": 668, "height": 402 } ]
{ "publication_title": "Density Functional Theory Study of Oxygen Adsorption on Polymer Surfaces for Atomic-Layer Etching: Implications for Semiconductor Device Fabrication", "authors": "Roberto C. Longo, Alok Ranjan, and Peter L. G. Ventzek*", "doi": null, "doi_candidates": [ "10.1021/acsanm.0c00618" ], ...
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Density Functional Theory Study of Oxygen Adsorption on Polymer Surfaces for Atomic-Layer Etching: Implications for Semiconductor Device Fabrication
Roberto C. Longo, Alok Ranjan, and Peter L. G. Ventzek*
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Density Functional Theory Study of Oxygen Adsorption on Polymer Surfaces for Atomic-Layer.pdf
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Figure 5. (a-d) Snapshots representing the $\mathrm{H}_2\mathrm{O}$ formation mechanism obtained in optimization of the $\mathrm{O}_5$ configuration, as shown in Figure 3 (the color code is the same). The left panel shows a complementary graph with relative energy along the formation pathway with respect to the ini...
sci_imageminer__atomic_layer_etching__simulation_usecase__35__fig5
atomic-layer-etching/simulation-usecase/35/FIG5
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{ "publication_title": "Density Functional Theory Study of Oxygen Adsorption on Polymer Surfaces for Atomic-Layer Etching: Implications for Semiconductor Device Fabrication", "authors": "Roberto C. Longo, Alok Ranjan, and Peter L. G. Ventzek*", "doi": null, "doi_candidates": [ "10.1021/acsanm.0c00618" ], ...
{ "extraction_method": "MinerU", "annotation_source": "Sci-ImageMiner per-image JSON", "classification_source": "repository_annotation_json", "content_source": "repository_content_json", "doi_extraction_method": null, "source_image_path": "train/atomic-layer-etching/simulation-usecase/35/images/FIG5.jpg", ...
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Density Functional Theory Study of Oxygen Adsorption on Polymer Surfaces for Atomic-Layer Etching: Implications for Semiconductor Device Fabrication
Roberto C. Longo, Alok Ranjan, and Peter L. G. Ventzek*
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Density Functional Theory Study of Oxygen Adsorption on Polymer Surfaces for Atomic-Layer.pdf
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0 Figure 6. Optimized geometries of one and two oxygen atoms adsorbed on partially dehydrogenated PS surfaces, expressed as a function of the hydrogen removal coverage $\theta$ . Brown, white, and red spheres represent carbon, hydrogen, and oxygen atoms, respectively.
sci_imageminer__atomic_layer_etching__simulation_usecase__35__fig6
atomic-layer-etching/simulation-usecase/35/FIG6
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[ { "panel_id": "a", "summary": "At low hydrogen coverage (θ(H) = 0.12), the optimized molecular structures remain relatively extended. The backbone shows limited bending, and the difference between the O and 2O configurations is modest, indicating minimal structural perturbation at this coverage." }, { ...
[ { "panel_id": "a", "data": "" }, { "panel_id": "b", "data": "" }, { "panel_id": "c", "data": "" }, { "panel_id": "d", "data": "" } ]
[ { "panel_id": "a", "question_type": "Process-Oriented", "question": "How does increasing hydrogen coverage affect the molecular structure in this figure?", "answer_type": "Paragraph", "answer": "At low hydrogen coverage, the molecular backbone remains relatively extended. As hydrogen coverage i...
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{ "publication_title": "Density Functional Theory Study of Oxygen Adsorption on Polymer Surfaces for Atomic-Layer Etching: Implications for Semiconductor Device Fabrication", "authors": "Roberto C. Longo, Alok Ranjan, and Peter L. G. Ventzek*", "doi": null, "doi_candidates": [ "10.1021/acsanm.0c00618" ], ...
{ "extraction_method": "MinerU", "annotation_source": "Sci-ImageMiner per-image JSON", "classification_source": "repository_annotation_json", "content_source": "repository_content_json", "doi_extraction_method": null, "source_image_path": "train/atomic-layer-etching/simulation-usecase/35/images/FIG6.jpg", ...
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Density Functional Theory Study of Oxygen Adsorption on Polymer Surfaces for Atomic-Layer Etching: Implications for Semiconductor Device Fabrication
Roberto C. Longo, Alok Ranjan, and Peter L. G. Ventzek*
null
null
2,020
Density Functional Theory Study of Oxygen Adsorption on Polymer Surfaces for Atomic-Layer.pdf
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Figure 7. (a-d) Snapshots representing the final configurations of oxygen adsorption on partially dehydrogenated PS, for a hydrogen removal coverage of $\theta = 0.48$ . The oxygen flux density and corresponding initial forces are listed below each picture. The graph shows the depth reached by the incoming oxygen atom...
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atomic-layer-etching/simulation-usecase/35/FIG7
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{ "publication_title": "Density Functional Theory Study of Oxygen Adsorption on Polymer Surfaces for Atomic-Layer Etching: Implications for Semiconductor Device Fabrication", "authors": "Roberto C. Longo, Alok Ranjan, and Peter L. G. Ventzek*", "doi": null, "doi_candidates": [ "10.1021/acsanm.0c00618" ], ...
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Density Functional Theory Study of Oxygen Adsorption on Polymer Surfaces for Atomic-Layer Etching: Implications for Semiconductor Device Fabrication
Roberto C. Longo, Alok Ranjan, and Peter L. G. Ventzek*
null
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Density Functional Theory Study of Oxygen Adsorption on Polymer Surfaces for Atomic-Layer.pdf
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Figure 1. Etch per cycle for TiN films versus $\mathrm{NbF}_5$ pulse time at $460^{\circ}C$ The duration of $\mathbb{N}_2$ purges and $\mathrm{CCl}_4$ pulses were fixed at 6 and 1 s, respectively.
sci_imageminer__atomic_layer_etching__simulation_usecase__4__figure_1
atomic-layer-etching/simulation-usecase/4/figure_1
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[ { "panel_id": "a", "label": "line chart" } ]
[ { "panel_id": "a", "summary": "The figure illustrates how the etch per cycle of TiN films varies with NbF₅ pulse time during the NbF₅–CCl₄ etch process at 460 °C. The etch per cycle increases from about 0.3 Å without NbF₅ to approximately 0.8 Å at a 3 s NbF₅ pulse, showing a gradual increase without clear s...
[ { "panel_id": "a", "data": "| NbF₅ pulse time [s] | Etch per cycle [Å] |\n|---|---|\n| 0.0 | 0.3 |\n| 1.0 | 0.6 |\n| 3.0 | 0.8 |" } ]
[ { "panel_id": "a", "question_type": "Process-Oriented", "question": "Is CCl₄ alone capable of etching TiN films at 460 °C without the use of NbF₅?", "answer_type": "Yes/No", "answer": "Yes" }, { "panel_id": "a", "question_type": "Comparative/Trend", "question": "How does the etch...
[ { "panel_id": "a", "x": 5, "y": 1, "width": 623, "height": 569 } ]
{ "publication_title": "Combining Experimental and DFT Investigation of the Mechanism Involved in Thermal Etching of Titanium Nitride Using Alternate Exposures of $\\mathrm{NbF}_5$ and $\\mathrm{CCl}_4$ , or $\\mathrm{CCl}_4$ Only", "authors": "Varun Sharma,\\* Suresh Kondati Natarajan, Simon D. Elliott, Tom B...
{ "extraction_method": "MinerU", "annotation_source": "Sci-ImageMiner per-image JSON", "classification_source": "repository_annotation_json", "content_source": "repository_content_json", "doi_extraction_method": null, "source_image_path": "train/atomic-layer-etching/simulation-usecase/4/images/figure_1.jpg"...
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Combining Experimental and DFT Investigation of the Mechanism Involved in Thermal Etching of Titanium Nitride Using Alternate Exposures of $\mathrm{NbF}_5$ and $\mathrm{CCl}_4$ , or $\mathrm{CCl}_4$ Only
Varun Sharma,\* Suresh Kondati Natarajan, Simon D. Elliott, Tom Blomberg, Suvi Haukka, Michael E. Givens, Marko Tuominen, and Mikko Ritala\*
null
null
null
Combining Experimental and DFT Investigation.pdf
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Figure 2. Etch per cycle of TiN films with varying $\mathbb{C}\mathbb{C}\mathbb{I}_4$ pulse time at $460^{\circ}C$ 6 s long $\mathbb{N}_2$ purges were used. The figure compares the EPC for the binary process (red) to the CVE process (blue).
sci_imageminer__atomic_layer_etching__simulation_usecase__4__figure_2
atomic-layer-etching/simulation-usecase/4/figure_2
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[ { "panel_id": "a", "label": "multiple line chart" } ]
[ { "panel_id": "a", "summary": "Figure 2 illustrates the etch per cycle (EPC) of TiN films as a function of CCl₄ pulse time at 460 °C, comparing two etching processes: the NbF₅–CCl₄ binary process and the CCl₄-only CVE process. The EPC increases with CCl₄ pulse time for both processes, with the binary proces...
[ { "panel_id": "a", "data": "| CCl₄ pulse time [s] | Etch per cycle NbF₅–CCl₄ [Å] | Etch per cycle CCl₄-only CVE [Å] |\n|---|---|---|\n| 0.0 | 0.0 | 0.0 |\n| 0.5 | 0.3 | 0.3 |\n| 1.0 | 0.4 | 0.4 |\n| 3.0 | 0.8 | 0.5 |" } ]
[ { "panel_id": "a", "question_type": "Process-Oriented", "question": "Can NbF₅ alone etch TiN films at 460 °C during the CCl₄ pulse experiments?", "answer_type": "Yes/No", "answer": "No" }, { "panel_id": "a", "question_type": "Comparative/Trend", "question": "How does the etch per...
[ { "panel_id": "a", "x": 6, "y": 4, "width": 624, "height": 595 } ]
{ "publication_title": "Combining Experimental and DFT Investigation of the Mechanism Involved in Thermal Etching of Titanium Nitride Using Alternate Exposures of $\\mathrm{NbF}_5$ and $\\mathrm{CCl}_4$ , or $\\mathrm{CCl}_4$ Only", "authors": "Varun Sharma,\\* Suresh Kondati Natarajan, Simon D. Elliott, Tom B...
{ "extraction_method": "MinerU", "annotation_source": "Sci-ImageMiner per-image JSON", "classification_source": "repository_annotation_json", "content_source": "repository_content_json", "doi_extraction_method": null, "source_image_path": "train/atomic-layer-etching/simulation-usecase/4/images/figure_2.jpg"...
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Combining Experimental and DFT Investigation of the Mechanism Involved in Thermal Etching of Titanium Nitride Using Alternate Exposures of $\mathrm{NbF}_5$ and $\mathrm{CCl}_4$ , or $\mathrm{CCl}_4$ Only
Varun Sharma,\* Suresh Kondati Natarajan, Simon D. Elliott, Tom Blomberg, Suvi Haukka, Michael E. Givens, Marko Tuominen, and Mikko Ritala\*
null
null
null
Combining Experimental and DFT Investigation.pdf
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Figure 3. Effect of etch temperature on etch per cycle for the binary process (blue curve) as well as $\mathrm{CCl_4}$ alone (blue curve) process. Both the precursor pulses and the purge times were fixed to 1 and 6 s, respectively.
sci_imageminer__atomic_layer_etching__simulation_usecase__4__figure_3
atomic-layer-etching/simulation-usecase/4/figure_3
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[ { "panel_id": "a", "label": "multiple line chart" } ]
[ { "panel_id": "a", "summary": "Figure 3 shows the effect of etch temperature on the etch per cycle of TiN films for the NbF₅–CCl₄ binary process and the CCl₄-only process. The etch per cycle increases with temperature for both processes, with the binary process consistently exhibiting higher etch rates. No ...
[ { "panel_id": "a", "data": "| Etch temperature [°C] | Etch per cycle NbF₅–CCl₄ [Å] | Etch per cycle CCl₄-only [Å] |\n|---|---|---|\n| 370 | 0.03 | 0.07 |\n| 380 | 0.10 | 0.12 |\n| 390 | 0.20 | 0.18 |\n| 400 | 0.40 | 0.22 |\n| 460 | 0.55 | 0.30 |" } ]
[ { "panel_id": "a", "question_type": "Process-Oriented", "question": "Can TiN films be etched significantly at temperatures below 370 °C for either the NbF₅–CCl₄ or CCl₄-only process?", "answer_type": "Yes/No", "answer": "No" }, { "panel_id": "a", "question_type": "Comparative/Trend",...
[ { "panel_id": "a", "x": 5, "y": 4, "width": 633, "height": 589 } ]
{ "publication_title": "Combining Experimental and DFT Investigation of the Mechanism Involved in Thermal Etching of Titanium Nitride Using Alternate Exposures of $\\mathrm{NbF}_5$ and $\\mathrm{CCl}_4$ , or $\\mathrm{CCl}_4$ Only", "authors": "Varun Sharma,\\* Suresh Kondati Natarajan, Simon D. Elliott, Tom B...
{ "extraction_method": "MinerU", "annotation_source": "Sci-ImageMiner per-image JSON", "classification_source": "repository_annotation_json", "content_source": "repository_content_json", "doi_extraction_method": null, "source_image_path": "train/atomic-layer-etching/simulation-usecase/4/images/figure_3.jpg"...
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Combining Experimental and DFT Investigation of the Mechanism Involved in Thermal Etching of Titanium Nitride Using Alternate Exposures of $\mathrm{NbF}_5$ and $\mathrm{CCl}_4$ , or $\mathrm{CCl}_4$ Only
Varun Sharma,\* Suresh Kondati Natarajan, Simon D. Elliott, Tom Blomberg, Suvi Haukka, Michael E. Givens, Marko Tuominen, and Mikko Ritala\*
null
null
null
Combining Experimental and DFT Investigation.pdf
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Figure 4. A change in the thickness values with total number of etch cycles at $460^{\circ}\mathrm{C}$ for TiN, $\mathrm{SiO_2}$ , $\mathrm{Al}_2\mathrm{O}_3$ , and $\mathrm{Si}_3\mathrm{N}_4$ films. A TiN is selectively etched away by $\mathrm{CCl_4}$ alone over other materials.
sci_imageminer__atomic_layer_etching__simulation_usecase__4__figure_4
atomic-layer-etching/simulation-usecase/4/figure_4
train
materials_science
atomic_layer_etching
null
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[ { "panel_id": "a", "label": "multiple line chart" } ]
[ { "panel_id": "a", "summary": "Figure 4 shows the change in film thickness with the total number of etch cycles at 460 °C for TiN, SiO₂, Al₂O₃, and Si₃N₄ films. The TiN film is selectively etched by the CCl₄-only CVE process, with thickness decreasing linearly at approximately 0.3 Å per cycle, reaching abou...
[ { "panel_id": "a", "data": "| Etch cycles | TiN (ALD) | Al₂O₃ (ALD) | SiO₂ (TOx) | Si₃N₄ (LPCVD) |\n|---|---|---|---|---|\n| 0 | 0 | 0 | 0 | 0 |\n| 100 | 3 | 0 | 0 | 0 |\n| 300 | 9 | 0 | 0 | 0 |\n| 500 | 13 | 0 | 0 | 0 |\n| 1000 | 30 | 0 | 0 | 0 |" } ]
[ { "panel_id": "a", "question_type": "Process-Oriented", "question": "Does the CCl₄-only CVE process etch Al₂O₃, SiO₂, or Si₃N₄ films at 460 °C?", "answer_type": "Yes/No", "answer": "no" }, { "panel_id": "a", "question_type": "Comparative/Trend", "question": "How does the thicknes...
[ { "panel_id": "a", "x": 2, "y": 3, "width": 618, "height": 567 } ]
{ "publication_title": "Combining Experimental and DFT Investigation of the Mechanism Involved in Thermal Etching of Titanium Nitride Using Alternate Exposures of $\\mathrm{NbF}_5$ and $\\mathrm{CCl}_4$ , or $\\mathrm{CCl}_4$ Only", "authors": "Varun Sharma,\\* Suresh Kondati Natarajan, Simon D. Elliott, Tom B...
{ "extraction_method": "MinerU", "annotation_source": "Sci-ImageMiner per-image JSON", "classification_source": "repository_annotation_json", "content_source": "repository_content_json", "doi_extraction_method": null, "source_image_path": "train/atomic-layer-etching/simulation-usecase/4/images/figure_4.jpg"...
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train/atomic-layer-etching/simulation-usecase/4/images/figure_4.json
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Combining Experimental and DFT Investigation of the Mechanism Involved in Thermal Etching of Titanium Nitride Using Alternate Exposures of $\mathrm{NbF}_5$ and $\mathrm{CCl}_4$ , or $\mathrm{CCl}_4$ Only
Varun Sharma,\* Suresh Kondati Natarajan, Simon D. Elliott, Tom Blomberg, Suvi Haukka, Michael E. Givens, Marko Tuominen, and Mikko Ritala\*
null
null
null
Combining Experimental and DFT Investigation.pdf
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Figure 5. An X-ray photoelectron spectroscopy of $\mathrm{SiO_2}$ surface after complete removal of TiN film by $\mathrm{CCl_4}$ based CVE process at $460^{\circ}\mathrm{C}$ .
sci_imageminer__atomic_layer_etching__simulation_usecase__4__figure_5
atomic-layer-etching/simulation-usecase/4/figure_5
train
materials_science
atomic_layer_etching
null
simulation
[ { "panel_id": "a", "label": "spectra chart" } ]
[ { "panel_id": "a", "summary": "Figure 5 shows an X-ray photoelectron spectroscopy (XPS) survey scan of the SiO₂ surface after complete removal of the TiN film by the CCl₄-based CVE process at 460 °C. The surface is primarily composed of silicon and oxygen, with small amounts of carbon (~5.1 at%) and nitroge...
[ { "panel_id": "a", "data": "| Binding energy [eV] | Element | Relative intensity [a.u.] |\n|---|---|---|\n| 284.8 | C 1s | Detected |\n| 399.1 | N 1s | Detected |\n| 532.0 | O 1s | Detected |\n| 103.3 | Si 2p | Detected |" } ]
[ { "panel_id": "a", "question_type": "Process-Oriented", "question": "Does the CCl₄-based CVE process at 460 °C completely remove the TiN film from the SiO₂ surface?", "answer_type": "Yes/No", "answer": "yes" }, { "panel_id": "a", "question_type": "Comparative/Trend", "question": ...
[ { "panel_id": "a", "x": 4, "y": 2, "width": 594, "height": 536 } ]
{ "publication_title": "Combining Experimental and DFT Investigation of the Mechanism Involved in Thermal Etching of Titanium Nitride Using Alternate Exposures of $\\mathrm{NbF}_5$ and $\\mathrm{CCl}_4$ , or $\\mathrm{CCl}_4$ Only", "authors": "Varun Sharma,\\* Suresh Kondati Natarajan, Simon D. Elliott, Tom B...
{ "extraction_method": "MinerU", "annotation_source": "Sci-ImageMiner per-image JSON", "classification_source": "repository_annotation_json", "content_source": "repository_content_json", "doi_extraction_method": null, "source_image_path": "train/atomic-layer-etching/simulation-usecase/4/images/figure_5.jpg"...
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Combining Experimental and DFT Investigation of the Mechanism Involved in Thermal Etching of Titanium Nitride Using Alternate Exposures of $\mathrm{NbF}_5$ and $\mathrm{CCl}_4$ , or $\mathrm{CCl}_4$ Only
Varun Sharma,\* Suresh Kondati Natarajan, Simon D. Elliott, Tom Blomberg, Suvi Haukka, Michael E. Givens, Marko Tuominen, and Mikko Ritala\*
null
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Combining Experimental and DFT Investigation.pdf
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Figure 6. BF-TEM images of a) the reference unetched $25 \text{nm}$ TiN film on $22 \text{nm} \text{SiO}_2$ film, b) after complete etching of $25 \text{nm}$ TiN film by 600 cycles of each $3 \text{s}$ long $\text{CCl}_4$ pulse separated by $6 \text{s}$ of $\text{N}_2$ purges.
sci_imageminer__atomic_layer_etching__simulation_usecase__4__figure_6
atomic-layer-etching/simulation-usecase/4/figure_6
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[ { "panel_id": "a", "summary": "BF-TEM image of the reference unetched TiN/SiO₂ system, showing a 25 nm TiN film on 22 nm SiO₂. Spin-on carbon was used to enhance material contrast." }, { "panel_id": "b", "summary": "BF-TEM image of the same sample after 600 cycles of 3 s CCl₄ pulses with 6 s N₂ ...
[ { "panel_id": "a", "data": "| Description |\n|---|\n| Reference unetched 25 nm TiN film on 22 nm SiO₂. Shows the original TiN layer for comparison. |" }, { "panel_id": "b", "data": "| Description |\n|---|\n| TiN film completely removed after 600 cycles of 3 s CCl₄ pulses with 6 s N₂ purges. The ...
[ { "panel_id": "a", "question_type": "Process-Oriented", "question": "Was the CCl₄-only CVE process effective in completely removing the TiN film from the SiO₂ surface?", "answer_type": "Yes/No", "answer": "Yes" }, { "panel_id": "a", "question_type": "Structure-Property", "questio...
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{ "publication_title": "Combining Experimental and DFT Investigation of the Mechanism Involved in Thermal Etching of Titanium Nitride Using Alternate Exposures of $\\mathrm{NbF}_5$ and $\\mathrm{CCl}_4$ , or $\\mathrm{CCl}_4$ Only", "authors": "Varun Sharma,\\* Suresh Kondati Natarajan, Simon D. Elliott, Tom B...
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Combining Experimental and DFT Investigation of the Mechanism Involved in Thermal Etching of Titanium Nitride Using Alternate Exposures of $\mathrm{NbF}_5$ and $\mathrm{CCl}_4$ , or $\mathrm{CCl}_4$ Only
Varun Sharma,\* Suresh Kondati Natarajan, Simon D. Elliott, Tom Blomberg, Suvi Haukka, Michael E. Givens, Marko Tuominen, and Mikko Ritala\*
null
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Combining Experimental and DFT Investigation.pdf
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Figure 7. An XPS depth profiling through remaining TiN film after partial etching at $460^{\circ} \text{C}$ . Total 300 cycles were performed with $0.5 \text{s}$ of both $\text{NbF}_5$ and $\text{CCl}_4$ pulse lengths with $6 \text{s}$ of $\text{N}_2$ purges.
sci_imageminer__atomic_layer_etching__simulation_usecase__4__figure_7
atomic-layer-etching/simulation-usecase/4/figure_7
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atomic_layer_etching
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[ { "panel_id": "a", "label": "multiple line chart" } ]
[ { "panel_id": "a", "summary": "Figure 7 presents an XPS depth profile of a partially etched TiN film after 300 cycles of the NbF₅–CCl₄ etch process at 460 °C, with 0.5 s pulses and 6 s N₂ purges. The surface initially contains high carbon (~26%) and oxygen (~31%), along with nitrogen (~20%), titanium (~15%)...
[ { "panel_id": "a", "data": "| Sputter time [s] | C1s (%) | N1s (%) | O1s (%) | F1s (%) | Si2p (%) | Ti2p (%) | Nb3d (%) |\n|---|---|---|---|---|---|---|---|\n| 0 | 26 | 20 | 31 | 1.5 | 1.5 | 15 | 5 |\n| 15 | 4 | 32 | 28 | 1.0 | 1.5 | 24 | 5.5 |\n| 60 | 3 | 32 | 28 | 0.9 | 1.5 | 24 | 6 |" } ]
[ { "panel_id": "a", "question_type": "Process-Oriented", "question": "Does the NbF₅–CCl₄ etch process at 460 °C cause incorporation of niobium and fluorine into the TiN film?", "answer_type": "Yes/No", "answer": "Yes" }, { "panel_id": "a", "question_type": "Comparative/Trend", "qu...
[ { "panel_id": "a", "x": 2, "y": 3, "width": 595, "height": 544 } ]
{ "publication_title": "Combining Experimental and DFT Investigation of the Mechanism Involved in Thermal Etching of Titanium Nitride Using Alternate Exposures of $\\mathrm{NbF}_5$ and $\\mathrm{CCl}_4$ , or $\\mathrm{CCl}_4$ Only", "authors": "Varun Sharma,\\* Suresh Kondati Natarajan, Simon D. Elliott, Tom B...
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Combining Experimental and DFT Investigation of the Mechanism Involved in Thermal Etching of Titanium Nitride Using Alternate Exposures of $\mathrm{NbF}_5$ and $\mathrm{CCl}_4$ , or $\mathrm{CCl}_4$ Only
Varun Sharma,\* Suresh Kondati Natarajan, Simon D. Elliott, Tom Blomberg, Suvi Haukka, Michael E. Givens, Marko Tuominen, and Mikko Ritala\*
null
null
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Combining Experimental and DFT Investigation.pdf
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Figure 8. Cross-sectional bright field transmission electron micrograph (BF-TEM) of 3D structures: a) about $3.3 \text{nm}$ TiN film deposited on $\text{SiO}_2$ fins with lateral cavities, b) the same after about $0.8 \text{nm}$ TiN is etched by the $\text{NbF}_5\text{-}\text{CCl}_4$ etch-process, and c) after ...
sci_imageminer__atomic_layer_etching__simulation_usecase__4__figure_8
atomic-layer-etching/simulation-usecase/4/figure_8
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[ { "panel_id": "a", "summary": "BF-TEM cross-section of pristine SiO₂ fin structures coated with a ~3.3 nm TiN layer, showing high conformality." }, { "panel_id": "b", "summary": "BF-TEM cross-section after partial etching (~0.8 nm) of the TiN layer using NbF₅–CCl₄ at 460 °C, showing minimal surf...
[ { "panel_id": "a", "data": "|Description|\n|-----------|\n| TEM image of SiO₂ fin structure coated with ~3.3 nm pristine TiN film, showing high conformality. |" }, { "panel_id": "b", "data": "|Description|\n|-----------|\n| TEM image after ~0.8 nm TiN conformally etched by the NbF₅–CCl₄ process,...
[ { "panel_id": "a", "question_type": "Process-Oriented", "question": "Does the NbF₅–CCl₄ etch process remove TiN conformally at 460 °C?", "answer_type": "Yes/No", "answer": "Yes" }, { "panel_id": "a", "question_type": "Comparative/Trend", "question": "Is the surface defect density...
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{ "publication_title": "Combining Experimental and DFT Investigation of the Mechanism Involved in Thermal Etching of Titanium Nitride Using Alternate Exposures of $\\mathrm{NbF}_5$ and $\\mathrm{CCl}_4$ , or $\\mathrm{CCl}_4$ Only", "authors": "Varun Sharma,\\* Suresh Kondati Natarajan, Simon D. Elliott, Tom B...
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Combining Experimental and DFT Investigation of the Mechanism Involved in Thermal Etching of Titanium Nitride Using Alternate Exposures of $\mathrm{NbF}_5$ and $\mathrm{CCl}_4$ , or $\mathrm{CCl}_4$ Only
Varun Sharma,\* Suresh Kondati Natarajan, Simon D. Elliott, Tom Blomberg, Suvi Haukka, Michael E. Givens, Marko Tuominen, and Mikko Ritala\*
null
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Combining Experimental and DFT Investigation.pdf
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Fig. 1 DFT and Tersoff calculated energy change during $\mathrm{Cl}_g$ adsorption and desorption from $\mathrm{Ge_9Cl_{12}}$ cluster. Light green: Cl. Cyan: Ge. H(0,2) and H(0,3) marks the number of neighbour atoms $k$ of Cl and Ge type for the surface Ge atom, not including its neighbour atom $j$ . For example,...
sci_imageminer__atomic_layer_etching__simulation_usecase__5__fig_1
atomic-layer-etching/simulation-usecase/5/fig_1
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{ "publication_title": "Computational modelling of atomic layer etching of chlorinated germanium surfaces by argon†", "authors": "Cite this: Phys. Chem. Chem. Phys., 2019, 21, 5898", "doi": "10.1039/c9cp00125e", "doi_candidates": [ "10.1039/c9cp00125e" ], "url": "https://doi.org/10.1039/c9cp00125e", "...
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Computational modelling of atomic layer etching of chlorinated germanium surfaces by argon†
Cite this: Phys. Chem. Chem. Phys., 2019, 21, 5898
10.1039/c9cp00125e
https://doi.org/10.1039/c9cp00125e
2,019
Computational modelling of atomic layer etching of chlorinated germanium surfaces by argon.pdf
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Fig. 2 (a) Side view of Ge surface after chlorination with different energies. The layer thickness showing here is around $16\mathrm{\AA}$ . Non-adsorbed Cl/Cl $_2$ away from surface have been deleted. (b) System energy (including both kinetic and potential energy) after equilibration (error bar smaller than the symb...
sci_imageminer__atomic_layer_etching__simulation_usecase__5__fig_2
atomic-layer-etching/simulation-usecase/5/fig_2
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{ "publication_title": "Computational modelling of atomic layer etching of chlorinated germanium surfaces by argon†", "authors": "Cite this: Phys. Chem. Chem. Phys., 2019, 21, 5898", "doi": "10.1039/c9cp00125e", "doi_candidates": [ "10.1039/c9cp00125e" ], "url": "https://doi.org/10.1039/c9cp00125e", "...
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train/atomic-layer-etching/simulation-usecase/5/content.json
Computational modelling of atomic layer etching of chlorinated germanium surfaces by argon†
Cite this: Phys. Chem. Chem. Phys., 2019, 21, 5898
10.1039/c9cp00125e
https://doi.org/10.1039/c9cp00125e
2,019
Computational modelling of atomic layer etching of chlorinated germanium surfaces by argon.pdf
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Fig. 3 Snapshots of Ge surface after $100\mathrm{eV}$ Ar bombardment (200 times). Light green: Cl. Cyan: Ge.
sci_imageminer__atomic_layer_etching__simulation_usecase__5__fig_3
atomic-layer-etching/simulation-usecase/5/fig_3
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[ { "panel_id": "a", "label": "molecular structure diagram" } ]
[]
[]
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[ { "panel_id": "a", "x": 4, "y": 6, "width": 600, "height": 288 } ]
{ "publication_title": "Computational modelling of atomic layer etching of chlorinated germanium surfaces by argon†", "authors": "Cite this: Phys. Chem. Chem. Phys., 2019, 21, 5898", "doi": "10.1039/c9cp00125e", "doi_candidates": [ "10.1039/c9cp00125e" ], "url": "https://doi.org/10.1039/c9cp00125e", "...
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Computational modelling of atomic layer etching of chlorinated germanium surfaces by argon†
Cite this: Phys. Chem. Chem. Phys., 2019, 21, 5898
10.1039/c9cp00125e
https://doi.org/10.1039/c9cp00125e
2,019
Computational modelling of atomic layer etching of chlorinated germanium surfaces by argon.pdf
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Fig. 5 (a) Density profile of Ge and Cl element change before and after 200 times Ar bombardment with different bombardment energy on $25\mathrm{eV}$ chlorinated surface. (b) Total etched number change (blue: Ge, red: Cl) with Ar bombardment energy for each chlorination condition, averaged from three samples with err...
sci_imageminer__atomic_layer_etching__simulation_usecase__5__fig_5
atomic-layer-etching/simulation-usecase/5/fig_5
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materials_science
atomic_layer_etching
null
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[ { "panel_id": "a", "label": "multiple line chart" }, { "panel_id": "b", "label": "multiple line chart" }, { "panel_id": "c", "label": "multiple line chart" }, { "panel_id": "d", "label": "multiple line chart" }, { "panel_id": "e", "label": "multiple line chart...
[ { "panel_id": "a", "summary": "The line chart shows the number density of Ge and Cl atoms at different z distances for initial and final states on 25 eV chlorinated surface." }, { "panel_id": "b", "summary": "The line chart shows the number density of Ge and Cl atoms at different z distances for...
[ { "panel_id": "a", "data": "| z distance (Å) | Density Ge_initial | Density Cl_initial | Density Ge_final | Density Cl_final |\n|---|---|---|---|---|\n| 0 | 0 | 0 | 0 | 0 |\n| 50 | 75 | 75 | 65 | 50 |" }, { "panel_id": "b", "data": "| z distance (Å) | Density Ge_initial | Density Cl_initial | De...
[ { "panel_id": "a", "question_type": "Comparative/Trend", "question": "How does the threshold bombardment energy for the onset of etching change with increasing chlorination energy (a through d)?", "answer_type": "Factoid", "answer": "The threshold energy decreases as the chlorination energy incr...
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{ "publication_title": "Computational modelling of atomic layer etching of chlorinated germanium surfaces by argon†", "authors": "Cite this: Phys. Chem. Chem. Phys., 2019, 21, 5898", "doi": "10.1039/c9cp00125e", "doi_candidates": [ "10.1039/c9cp00125e" ], "url": "https://doi.org/10.1039/c9cp00125e", "...
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Computational modelling of atomic layer etching of chlorinated germanium surfaces by argon†
Cite this: Phys. Chem. Chem. Phys., 2019, 21, 5898
10.1039/c9cp00125e
https://doi.org/10.1039/c9cp00125e
2,019
Computational modelling of atomic layer etching of chlorinated germanium surfaces by argon.pdf
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FIG.2. $\mathbb{C}\mathbb{I}_2$ mass flow, pressure, and DC bias during one 7 s ALE cycle. The applied DC bias is $-65\mathrm{V}$ for this case. The Ar flow (80 SCCM) is on continuously throughout the cycle. ICP power is 250 W.
sci_imageminer__atomic_layer_etching__simulation_usecase__6__fig2
atomic-layer-etching/simulation-usecase/6/fig2
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[ { "panel_id": "a", "label": "multiple line chart" } ]
[ { "panel_id": "a", "summary": "The multi-axis chart shows the evolution of DC self-bias voltage, chlorine gas flow, and chamber pressure over time. The process is divided into four clearly marked steps, each showing how plasma conditions and gas flow influence system parameters. The other panels are not sep...
[ { "panel_id": "a", "data": "| Time (s) | DC Self-Bias (V) | Cl₂ Flow (seccm) | P (mTorr) |\n|----------|------------------|------------------|-----------|\n| 0 | 0 | 0 | 22 |\n| 1 | 0 | 20 | 22 |\n| 2 | -60 ...
[ { "panel_id": "a", "question_type": "Process-Oriented", "question": "What are the four steps shown in the figure?", "answer_type": "List", "answer": "Step 1: Cl₂ On, ICP Off, Bias Off; Step 2: ICP On, Bias On; Step 3: Cl₂ Off, Bias Off; Step 4: All Off" }, { "panel_id": "a", "questio...
[ { "panel_id": "a", "x": 0, "y": 0, "width": 678, "height": 475 } ]
{ "publication_title": "Dynamics of plasma atomic layer etching: Molecular dynamics simulations and optical emission spectroscopy", "authors": "Special Collection: Atomic Layer Etching (ALE)", "doi": "10.1116/S00003011.1", "doi_candidates": [ "10.1116/S00003011.1", "10.1116/s0003011", "10.1116/6.000...
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Dynamics of plasma atomic layer etching: Molecular dynamics simulations and optical emission spectroscopy
Special Collection: Atomic Layer Etching (ALE)
10.1116/S00003011.1
https://doi.org/10.1116/S00003011.1
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Dynamics of plasma atomic layer etching Molecular.pdf
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FIG. 1. Schematic of the experimental apparatus. The plasma is powered by an inductively coupled coil at the top and by a RF biased substrate stage. The major measurements are of the etch rate (via laser interferometry) and optical emission spectroscopy of species near the silicon substrate being etched during the $\m...
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atomic-layer-etching/simulation-usecase/6/fig_1
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{ "publication_title": "Dynamics of plasma atomic layer etching: Molecular dynamics simulations and optical emission spectroscopy", "authors": "Special Collection: Atomic Layer Etching (ALE)", "doi": "10.1116/S00003011.1", "doi_candidates": [ "10.1116/S00003011.1", "10.1116/s0003011", "10.1116/6.000...
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Dynamics of plasma atomic layer etching: Molecular dynamics simulations and optical emission spectroscopy
Special Collection: Atomic Layer Etching (ALE)
10.1116/S00003011.1
https://doi.org/10.1116/S00003011.1
2,023
Dynamics of plasma atomic layer etching Molecular.pdf
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1.0.0
FIG. 10. OES signals for atomic Si (bottom line), SiCl (top line), and $\mathrm{SiCl_2}$ (middle line) for $80\mathrm{eVAr^{+}}$ Results are shown for two ALE cycles. The signal for SiCl is multiplied by 10 and the signal for $\mathrm{SiCl_2}$ is multiplied by 100. The atomic Si signal is modified to account for ...
sci_imageminer__atomic_layer_etching__simulation_usecase__6__fig_10
atomic-layer-etching/simulation-usecase/6/fig_10
train
materials_science
atomic_layer_etching
null
simulation
[ { "panel_id": "a", "label": "multi spectra chart" } ]
[ { "panel_id": "a", "summary": "The figure displays a multiple line chart showing the temporal evolution of product counts for Si, SiCl, and SiCl₂ during a repeated four-step process. Product counts peak during specific steps and return to baseline in others, demonstrating step-dependent product formation." ...
[ { "panel_id": "a", "data": "| Time (s) | Product Count (arb. units) |\n|---|---|\n| 0 | 0 |\n| 5 | 0 |\n| 10 | 0 |\n| 15 | 0 |\n| 20 | 0 |\n| 25 | 0 |\n| 30 | 0 |\n| 35 | 0 |\n| 40 | 0 |\n| 45 | 0 |\n| 50 | 0 |\n| 55 | 0 |\n| 60 | 0 |\n| 65 | 0 |\n| 70 | 0 |\n| 75 | 0 |\n| 80 | 0 |\n| 85 | 0 |\n| 90 | 0 |\n...
[ { "panel_id": "a", "question_type": "Comparative/Trend", "question": "What trend is observed across Steps 1 to 4 during each cycle?", "answer_type": "Paragraph", "answer": "The graph shows a clear cyclic pattern in product count behavior across Steps 1 through 4. During Step 1, all product speci...
[ { "panel_id": "a", "x": 0, "y": 0, "width": 678, "height": 470 } ]
{ "publication_title": "Dynamics of plasma atomic layer etching: Molecular dynamics simulations and optical emission spectroscopy", "authors": "Special Collection: Atomic Layer Etching (ALE)", "doi": "10.1116/S00003011.1", "doi_candidates": [ "10.1116/S00003011.1", "10.1116/s0003011", "10.1116/6.000...
{ "extraction_method": "MinerU", "annotation_source": "Sci-ImageMiner per-image JSON", "classification_source": "repository_annotation_json", "content_source": "repository_content_json", "doi_extraction_method": "page0_regex", "source_image_path": "train/atomic-layer-etching/simulation-usecase/6/images/fig_...
train/atomic-layer-etching/simulation-usecase/6/images/fig_10.jpg
train/atomic-layer-etching/simulation-usecase/6/images/fig_10.json
train/atomic-layer-etching/simulation-usecase/6/content.json
Dynamics of plasma atomic layer etching: Molecular dynamics simulations and optical emission spectroscopy
Special Collection: Atomic Layer Etching (ALE)
10.1116/S00003011.1
https://doi.org/10.1116/S00003011.1
2,023
Dynamics of plasma atomic layer etching Molecular.pdf
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1.0.0
FIG. 11. Si OES modified to account for dissociative excitation of SiCl as a function of time for various $\mathrm{Ar^{+}}$ energies. Results are shown for two ALE cycles. The top line corresponds to results for $215\mathrm{eV}$ , the middle line for $80\mathrm{eV}$ , and the bottom line for $45\mathrm{eV}$ .
sci_imageminer__atomic_layer_etching__simulation_usecase__6__fig_11
atomic-layer-etching/simulation-usecase/6/fig_11
train
materials_science
atomic_layer_etching
null
simulation
[ { "panel_id": "a", "label": "multi spectra chart" } ]
[ { "panel_id": "a", "summary": "The figure presents a multi-line plot showing product count (in arbitrary units) over time for three different incident electron energies: 45 eV, 80 eV, and 215 eV. Each energy condition produces a distinct response pattern across four repeated steps, with the 215 eV trace sho...
[ { "panel_id": "a", "data": "| Time (s) | 45 eV | 80 eV | 215 eV |\n|----------|--------|--------|---------|\n| 0 | 0 | 0 | 0 |\n| 1 | ~20k | ~60k | ~180k |\n| 2 | ~20k | ~60k | ~180k |\n| 5 | ~20k | ~60k | ~180k |\n| 6 | 0 | 0 ...
[ { "panel_id": "a", "question_type": "Comparative/Trend", "question": "Does the prodcut count increase with increasing energy level across all time steps?", "answer_type": "Yes/No", "answer": "Yes" }, { "panel_id": "a", "question_type": "Structure-Property", "question": "At which ...
[ { "panel_id": "a", "x": 0, "y": 0, "width": 669, "height": 458 } ]
{ "publication_title": "Dynamics of plasma atomic layer etching: Molecular dynamics simulations and optical emission spectroscopy", "authors": "Special Collection: Atomic Layer Etching (ALE)", "doi": "10.1116/S00003011.1", "doi_candidates": [ "10.1116/S00003011.1", "10.1116/s0003011", "10.1116/6.000...
{ "extraction_method": "MinerU", "annotation_source": "Sci-ImageMiner per-image JSON", "classification_source": "repository_annotation_json", "content_source": "repository_content_json", "doi_extraction_method": "page0_regex", "source_image_path": "train/atomic-layer-etching/simulation-usecase/6/images/fig_...
train/atomic-layer-etching/simulation-usecase/6/images/fig_11.jpg
train/atomic-layer-etching/simulation-usecase/6/images/fig_11.json
train/atomic-layer-etching/simulation-usecase/6/content.json
Dynamics of plasma atomic layer etching: Molecular dynamics simulations and optical emission spectroscopy
Special Collection: Atomic Layer Etching (ALE)
10.1116/S00003011.1
https://doi.org/10.1116/S00003011.1
2,023
Dynamics of plasma atomic layer etching Molecular.pdf
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FIG. 12. Normalized atomic Si counts as a function of $\mathsf{Ar}^+$ fluence for various $\mathsf{Ar}^+$ energies. Subfigure (a) shows the results for OES experiments (using the modified OES Si signals) and subfigure (b) shows results from MD ALE simulations. For both the OES and MD results, the counts are normali...
sci_imageminer__atomic_layer_etching__simulation_usecase__6__fig_12
atomic-layer-etching/simulation-usecase/6/fig_12
train
materials_science
atomic_layer_etching
null
simulation
[ { "panel_id": "a", "label": "multiple scatter plot" }, { "panel_id": "b", "label": "multiple scatter plot" } ]
[ { "panel_id": "a", "summary": "Panel (a) shows experimental measurements of Si count as a function of Ar⁺ ion dosage for three incident energies. The Si signal is consistently highest at 215 eV and increases with dosage before saturating, while the 80 eV signal shows a moderate rise and 45 eV shows negligib...
[ { "panel_id": "a", "data": "| Ion Dosage (Ar⁺/cm²) × 10¹⁵ | 45 eV | 80 eV | 215 eV |\n|----------------------------|-------|-------|--------|\n| 0 | 0 | 0 | 2 |\n| 10 | 0 | 0.5 | 4 |\n| 20 | 0 | 1 | 5 ...
[ { "panel_id": "a", "question_type": "Comparative/Trend", "question": "Does the Si count at 215 eV p,ateau after an ion dosage of approximately 30 × 10¹⁵ Ar⁺/cm² in both experiment and simulation?", "answer_type": "Yes/No", "answer": "Yes" }, { "panel_id": "a", "question_type": "Proce...
[ { "panel_id": "a", "x": 8, "y": 2, "width": 679, "height": 458 }, { "panel_id": "b", "x": 721, "y": 3, "width": 687, "height": 457 } ]
{ "publication_title": "Dynamics of plasma atomic layer etching: Molecular dynamics simulations and optical emission spectroscopy", "authors": "Special Collection: Atomic Layer Etching (ALE)", "doi": "10.1116/S00003011.1", "doi_candidates": [ "10.1116/S00003011.1", "10.1116/s0003011", "10.1116/6.000...
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train/atomic-layer-etching/simulation-usecase/6/images/fig_12.jpg
train/atomic-layer-etching/simulation-usecase/6/images/fig_12.json
train/atomic-layer-etching/simulation-usecase/6/content.json
Dynamics of plasma atomic layer etching: Molecular dynamics simulations and optical emission spectroscopy
Special Collection: Atomic Layer Etching (ALE)
10.1116/S00003011.1
https://doi.org/10.1116/S00003011.1
2,023
Dynamics of plasma atomic layer etching Molecular.pdf
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FIG. 13. Normalized SiCl counts as a function of $\mathsf{Ar}^+$ fluence for various $\mathsf{Ar}^+$ energies. Subfigure (a) shows the results for OES experiments and subfigure (b) shows results from MD ALE simulations. For both the OES and MD results, the counts are normalized using the value at the peak observed ...
sci_imageminer__atomic_layer_etching__simulation_usecase__6__fig_13
atomic-layer-etching/simulation-usecase/6/fig_13
train
materials_science
atomic_layer_etching
null
simulation
[ { "panel_id": "a", "label": "multiple scatter plot" }, { "panel_id": "b", "label": "multiple scatter plot" } ]
[ { "panel_id": "a", "summary": "The pair of scatter plots show the experimental (left) and MD-simulated (right) SiCl count as a function of Ar⁺ ion dosage for three ion energies: 45 eV, 80 eV, and 215 eV. In both cases, the SiCl count decreases with increasing dosage, with the highest initial counts observed...
[ { "panel_id": "a", "data": "| Ion Dosage (Ar<sup>+</sup>/cm<sup>2</sup>) × 10<sup>15</sup> | 45 eV | 80 eV | 215 eV |\n|---|---|---|---|\n| 0 | 0.75 | 0.90 | 1.60 |\n| 5 | 0.60 | 0.70 | 0.80 |\n| 10 | 0.55 | 0.60 | 0.70 |\n| 15 | 0.50 | 0.55 | 0.60 |\n| 20 | 0.45 | 0.50 | 0.55 |\n| 25 | 0.40 | 0.45 | 0.50 |...
[ { "panel_id": "a", "question_type": "Comparative/Trend", "question": "Does the SiCl count decrease with increasing ion dosage for all energies in both experiment and simulation?", "answer_type": "Yes/No", "answer": "Yes" }, { "panel_id": "a", "question_type": "Structure-Property", ...
[ { "panel_id": "a", "x": 10, "y": 10, "width": 682, "height": 448 }, { "panel_id": "b", "x": 725, "y": 10, "width": 686, "height": 448 } ]
{ "publication_title": "Dynamics of plasma atomic layer etching: Molecular dynamics simulations and optical emission spectroscopy", "authors": "Special Collection: Atomic Layer Etching (ALE)", "doi": "10.1116/S00003011.1", "doi_candidates": [ "10.1116/S00003011.1", "10.1116/s0003011", "10.1116/6.000...
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train/atomic-layer-etching/simulation-usecase/6/images/fig_13.jpg
train/atomic-layer-etching/simulation-usecase/6/images/fig_13.json
train/atomic-layer-etching/simulation-usecase/6/content.json
Dynamics of plasma atomic layer etching: Molecular dynamics simulations and optical emission spectroscopy
Special Collection: Atomic Layer Etching (ALE)
10.1116/S00003011.1
https://doi.org/10.1116/S00003011.1
2,023
Dynamics of plasma atomic layer etching Molecular.pdf
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FIG. 14. Normalized $\mathrm{SiCl}_2$ counts as a function of $\mathsf{Ar}^+$ fluence for various $\mathsf{Ar}^+$ energies. Subfigure (a) shows the results for OES experiments and subfigure (b) shows results from MD ALE simulations. For both the OES and MD results, the counts are normalized using the value at the...
sci_imageminer__atomic_layer_etching__simulation_usecase__6__fig_14
atomic-layer-etching/simulation-usecase/6/fig_14
train
materials_science
atomic_layer_etching
null
simulation
[ { "panel_id": "a", "label": "multiple scatter plot" }, { "panel_id": "b", "label": "multiple scatter plot" } ]
[ { "panel_id": "a", "summary": "The experimental scatter plot shows that the SiCl₂ count decreases as ion dosage increases for all energy levels (45 eV, 80 eV, 215 eV). The highest counts are seen at 215 eV, while the lowest are at 45 eV. After ~30×10¹⁵ Ar⁺/cm², the counts plateau, indicating a saturation or...
[ { "panel_id": "a", "data": "| Ion Dosage (Ar⁺/cm²) × 10¹⁵ | 45 eV | 80 eV | 215 eV |\n|-----------------------------|--------|--------|---------|\n| 0 | 1.2 | 1.4 | 1.6 |\n| 5 | 0.9 | 1.1 | 1.3 |\n| 10 | 0.7 ...
[ { "panel_id": "a", "question_type": "Comparative/Trend", "question": "How does SiCl₂ count vary with increasing ion dosage in both experiment and simulation, and how does this vary with ion energy?", "answer_type": "Paragraph", "answer": "In both experimental and simulated datasets, the SiCl₂ co...
[ { "panel_id": "a", "x": 9, "y": 10, "width": 683, "height": 451 }, { "panel_id": "b", "x": 725, "y": 9, "width": 684, "height": 452 } ]
{ "publication_title": "Dynamics of plasma atomic layer etching: Molecular dynamics simulations and optical emission spectroscopy", "authors": "Special Collection: Atomic Layer Etching (ALE)", "doi": "10.1116/S00003011.1", "doi_candidates": [ "10.1116/S00003011.1", "10.1116/s0003011", "10.1116/6.000...
{ "extraction_method": "MinerU", "annotation_source": "Sci-ImageMiner per-image JSON", "classification_source": "repository_annotation_json", "content_source": "repository_content_json", "doi_extraction_method": "page0_regex", "source_image_path": "train/atomic-layer-etching/simulation-usecase/6/images/fig_...
train/atomic-layer-etching/simulation-usecase/6/images/fig_14.jpg
train/atomic-layer-etching/simulation-usecase/6/images/fig_14.json
train/atomic-layer-etching/simulation-usecase/6/content.json
Dynamics of plasma atomic layer etching: Molecular dynamics simulations and optical emission spectroscopy
Special Collection: Atomic Layer Etching (ALE)
10.1116/S00003011.1
https://doi.org/10.1116/S00003011.1
2,023
Dynamics of plasma atomic layer etching Molecular.pdf
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FIG. 15. Normalized atomic Cl counts as a function of $\mathsf{Ar}^+$ fluence. Subfigure (a) shows the results for OES experiments (where the ion energy is estimated to be about $85\mathrm{eV}$ ) and subfigure (b) shows results from MD ALE simulations where the ion energy is $80\mathrm{eV}$ . In both cases, the res...
sci_imageminer__atomic_layer_etching__simulation_usecase__6__fig_15
atomic-layer-etching/simulation-usecase/6/fig_15
train
materials_science
atomic_layer_etching
null
simulation
[ { "panel_id": "a", "label": "scatter plot" }, { "panel_id": "b", "label": "box plot" } ]
[ { "panel_id": "a", "summary": "The experimental scatter plot shows a sharp decrease in Cl count with increasing ion dosage up to about 10–15 × 10¹⁵ Ar⁺/cm². After that, the count levels off around 0.5 arb. units, suggesting that most Cl atoms have been desorbed or sputtered and that the system has reached a...
[ { "panel_id": "a", "data": "| Ion Dosage (Ar⁺/cm²) × 10¹⁵ | Cl Count (arb. units) |\n|-----------------------------|------------------------|\n| 0 | 1.20 |\n| 2 | 1.00 |\n| 4 | 0.90 ...
[ { "panel_id": "a", "question_type": "Process-Oriented", "question": "How does the Cl coynt vary with increasing ion dosage in the experimental and simualtion plots?", "answer_type": "Paragraph", "answer": "In both the experimental and simulation results, Cl count decreases as ion dosage increase...
[ { "panel_id": "a", "x": 8, "y": 11, "width": 686, "height": 478 }, { "panel_id": "b", "x": 720, "y": 7, "width": 690, "height": 481 } ]
{ "publication_title": "Dynamics of plasma atomic layer etching: Molecular dynamics simulations and optical emission spectroscopy", "authors": "Special Collection: Atomic Layer Etching (ALE)", "doi": "10.1116/S00003011.1", "doi_candidates": [ "10.1116/S00003011.1", "10.1116/s0003011", "10.1116/6.000...
{ "extraction_method": "MinerU", "annotation_source": "Sci-ImageMiner per-image JSON", "classification_source": "repository_annotation_json", "content_source": "repository_content_json", "doi_extraction_method": "page0_regex", "source_image_path": "train/atomic-layer-etching/simulation-usecase/6/images/fig_...
train/atomic-layer-etching/simulation-usecase/6/images/fig_15.jpg
train/atomic-layer-etching/simulation-usecase/6/images/fig_15.json
train/atomic-layer-etching/simulation-usecase/6/content.json
Dynamics of plasma atomic layer etching: Molecular dynamics simulations and optical emission spectroscopy
Special Collection: Atomic Layer Etching (ALE)
10.1116/S00003011.1
https://doi.org/10.1116/S00003011.1
2,023
Dynamics of plasma atomic layer etching Molecular.pdf
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FIG. 3. Side views of the simulations cell at various values of $\mathsf{Ar}^+$ fluences during the ion bombardment step. The snapshot with the label of $0\mathrm{ML}$ of $\mathsf{Ar}^+$ refers to the simulation cell immediately after the chlorination step, before ion bombardment has begun. Translucent yellow sph...
sci_imageminer__atomic_layer_etching__simulation_usecase__6__fig_3
atomic-layer-etching/simulation-usecase/6/fig_3
train
materials_science
atomic_layer_etching
null
simulation
[ { "panel_id": "a", "label": "conceptual diagram" } ]
[]
[]
[]
[ { "panel_id": "a", "x": 0, "y": 0, "width": 536, "height": 919 } ]
{ "publication_title": "Dynamics of plasma atomic layer etching: Molecular dynamics simulations and optical emission spectroscopy", "authors": "Special Collection: Atomic Layer Etching (ALE)", "doi": "10.1116/S00003011.1", "doi_candidates": [ "10.1116/S00003011.1", "10.1116/s0003011", "10.1116/6.000...
{ "extraction_method": "MinerU", "annotation_source": "Sci-ImageMiner per-image JSON", "classification_source": "repository_annotation_json", "content_source": "repository_content_json", "doi_extraction_method": "page0_regex", "source_image_path": "train/atomic-layer-etching/simulation-usecase/6/images/fig_...
train/atomic-layer-etching/simulation-usecase/6/images/fig_3.jpg
train/atomic-layer-etching/simulation-usecase/6/images/fig_3.json
train/atomic-layer-etching/simulation-usecase/6/content.json
Dynamics of plasma atomic layer etching: Molecular dynamics simulations and optical emission spectroscopy
Special Collection: Atomic Layer Etching (ALE)
10.1116/S00003011.1
https://doi.org/10.1116/S00003011.1
2,023
Dynamics of plasma atomic layer etching Molecular.pdf
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1.0.0
FIG. 4. Top views of the simulations cell at various values of $\mathsf{Ar}^+$ fluences during the ion bombardment step corresponding to Fig. 3 (80 eV ion energy). The surface of the cell can be seen to be nearly saturated with $\mathrm{Cl}$ before ion bombardment has begun (i.e., $0\mathrm{ML}$ fluence). After ...
sci_imageminer__atomic_layer_etching__simulation_usecase__6__fig_4
atomic-layer-etching/simulation-usecase/6/fig_4
train
materials_science
atomic_layer_etching
null
simulation
[ { "panel_id": "a", "label": "conceptual diagram" } ]
[]
[]
[]
[ { "panel_id": "a", "x": 0, "y": 0, "width": 533, "height": 778 } ]
{ "publication_title": "Dynamics of plasma atomic layer etching: Molecular dynamics simulations and optical emission spectroscopy", "authors": "Special Collection: Atomic Layer Etching (ALE)", "doi": "10.1116/S00003011.1", "doi_candidates": [ "10.1116/S00003011.1", "10.1116/s0003011", "10.1116/6.000...
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train/atomic-layer-etching/simulation-usecase/6/images/fig_4.jpg
train/atomic-layer-etching/simulation-usecase/6/images/fig_4.json
train/atomic-layer-etching/simulation-usecase/6/content.json
Dynamics of plasma atomic layer etching: Molecular dynamics simulations and optical emission spectroscopy
Special Collection: Atomic Layer Etching (ALE)
10.1116/S00003011.1
https://doi.org/10.1116/S00003011.1
2,023
Dynamics of plasma atomic layer etching Molecular.pdf
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FIG. 5. Depiction of the near-surface phenomena during $\mathsf{Ar^+}$ bombardment in $\mathrm{Si - Cl_2 - Ar}$ ALE as observed in MD simulations. The regions labeled by red brackets and separated by red dashed lines are the Cl layer, amorphous mixed layer, and crystalline Si region. The green arrows indicate the m...
sci_imageminer__atomic_layer_etching__simulation_usecase__6__fig_5
atomic-layer-etching/simulation-usecase/6/fig_5
train
materials_science
atomic_layer_etching
null
simulation
[ { "panel_id": "a", "label": "conceptual diagram" } ]
[]
[]
[]
[ { "panel_id": "a", "x": 0, "y": 0, "width": 675, "height": 750 } ]
{ "publication_title": "Dynamics of plasma atomic layer etching: Molecular dynamics simulations and optical emission spectroscopy", "authors": "Special Collection: Atomic Layer Etching (ALE)", "doi": "10.1116/S00003011.1", "doi_candidates": [ "10.1116/S00003011.1", "10.1116/s0003011", "10.1116/6.000...
{ "extraction_method": "MinerU", "annotation_source": "Sci-ImageMiner per-image JSON", "classification_source": "repository_annotation_json", "content_source": "repository_content_json", "doi_extraction_method": "page0_regex", "source_image_path": "train/atomic-layer-etching/simulation-usecase/6/images/fig_...
train/atomic-layer-etching/simulation-usecase/6/images/fig_5.jpg
train/atomic-layer-etching/simulation-usecase/6/images/fig_5.json
train/atomic-layer-etching/simulation-usecase/6/content.json
Dynamics of plasma atomic layer etching: Molecular dynamics simulations and optical emission spectroscopy
Special Collection: Atomic Layer Etching (ALE)
10.1116/S00003011.1
https://doi.org/10.1116/S00003011.1
2,023
Dynamics of plasma atomic layer etching Molecular.pdf
fig_5
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FIG. 6. Amount of Si etched (in units of $\mathrm{A}$ ) (blue lines) and Cl uptake (red lines) as a function of cycle number for $\mathrm{Si - Cl_2 - Ar}$ ALE simulation using $100\mathrm{eV}$ $\mathrm{Ar^+}$ . One cycle consists of $28.2\mathrm{ML}$ of $\mathrm{Cl}_2$ molecule impacts and $28.2\mathrm{ML}$ o...
sci_imageminer__atomic_layer_etching__simulation_usecase__6__fig_6
atomic-layer-etching/simulation-usecase/6/fig_6
train
materials_science
atomic_layer_etching
null
simulation
[ { "panel_id": "a", "label": "multi-axis chart" } ]
[ { "panel_id": "a", "summary": "This multi-axis chart tracks the progression of Si etching and Cl uptake across five repeated cycles under 100 eV Ar⁺ ion bombardment. The red curve (left y-axis) indicates the amount of Si etched per cycle, which increases sharply during each ion bombardment step and then ret...
[ { "panel_id": "a", "data": "| Cycle Number | Si Etched (Å) | Cl Uptake (Cl/cm² × 10¹⁵) |\n|--------------|----------------|----------------------------|\n| 0 | 0 | 0.10 |\n| 1 | 32 | 0.22 |\n| 2 | 32 ...
[ { "panel_id": "a", "question_type": "Comparative/Trend", "question": "How do the trends of Si etching and Cl uptake differ across ALD/E cycles?", "answer_type": "Paragraph", "answer": "The Si etching profile exhibits a periodic, stepwise increase and reset pattern with each cycle, reflecting ion...
[ { "panel_id": "a", "x": 0, "y": 0, "width": 675, "height": 428 } ]
{ "publication_title": "Dynamics of plasma atomic layer etching: Molecular dynamics simulations and optical emission spectroscopy", "authors": "Special Collection: Atomic Layer Etching (ALE)", "doi": "10.1116/S00003011.1", "doi_candidates": [ "10.1116/S00003011.1", "10.1116/s0003011", "10.1116/6.000...
{ "extraction_method": "MinerU", "annotation_source": "Sci-ImageMiner per-image JSON", "classification_source": "repository_annotation_json", "content_source": "repository_content_json", "doi_extraction_method": "page0_regex", "source_image_path": "train/atomic-layer-etching/simulation-usecase/6/images/fig_...
train/atomic-layer-etching/simulation-usecase/6/images/fig_6.jpg
train/atomic-layer-etching/simulation-usecase/6/images/fig_6.json
train/atomic-layer-etching/simulation-usecase/6/content.json
Dynamics of plasma atomic layer etching: Molecular dynamics simulations and optical emission spectroscopy
Special Collection: Atomic Layer Etching (ALE)
10.1116/S00003011.1
https://doi.org/10.1116/S00003011.1
2,023
Dynamics of plasma atomic layer etching Molecular.pdf
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FIG. 7. Amount of Si etched in units of $\dot{A}$ (blue lines) and Cl uptake (red lines) during the final cycle for the $\mathrm{Si - Cl_2 - Ar}$ ALE simulation using $100\mathrm{eVAr^{+}}$ The final portion of the ion bombardment step (purple dashed-dotted line) is used to calculate the etch yield shown as the p...
sci_imageminer__atomic_layer_etching__simulation_usecase__6__fig_7
atomic-layer-etching/simulation-usecase/6/fig_7
train
materials_science
atomic_layer_etching
null
simulation
[ { "panel_id": "a", "label": "multi-axis chart" } ]
[ { "panel_id": "a", "summary": "This multi-axis chart illustrates the relationship between species dosage (Cl₂ or Ar⁺/cm²) and two parameters: Si etching depth and chlorine uptake. The red curve (left y-axis) represents silicon etching at 100 eV Ar⁺, which begins only after Cl₂ exposure has saturated the sur...
[ { "panel_id": "a", "data": "| Species Dosage (Cl₂ or Ar⁺/cm²) × 10¹⁵ | Si Etched (Å) | Cl Uptake (Cl/cm²) × 10¹⁵ |\n|----------------------------------------|---------------|----------------------------|\n| 0 | 0 | 0 |\n| 10 ...
[ { "panel_id": "a", "question_type": "Comparative/Trend", "question": "What do the trends in Si etching and Cl uptake differ as species dosage increases?", "answer_type": "Paragraph", "answer": "Chlorine uptake increases rapidly during initial Cl₂ exposure and saturates near 1.35 × 10¹⁵ Cl/cm², ...
[ { "panel_id": "a", "x": 0, "y": 0, "width": 669, "height": 425 } ]
{ "publication_title": "Dynamics of plasma atomic layer etching: Molecular dynamics simulations and optical emission spectroscopy", "authors": "Special Collection: Atomic Layer Etching (ALE)", "doi": "10.1116/S00003011.1", "doi_candidates": [ "10.1116/S00003011.1", "10.1116/s0003011", "10.1116/6.000...
{ "extraction_method": "MinerU", "annotation_source": "Sci-ImageMiner per-image JSON", "classification_source": "repository_annotation_json", "content_source": "repository_content_json", "doi_extraction_method": "page0_regex", "source_image_path": "train/atomic-layer-etching/simulation-usecase/6/images/fig_...
train/atomic-layer-etching/simulation-usecase/6/images/fig_7.jpg
train/atomic-layer-etching/simulation-usecase/6/images/fig_7.json
train/atomic-layer-etching/simulation-usecase/6/content.json
Dynamics of plasma atomic layer etching: Molecular dynamics simulations and optical emission spectroscopy
Special Collection: Atomic Layer Etching (ALE)
10.1116/S00003011.1
https://doi.org/10.1116/S00003011.1
2,023
Dynamics of plasma atomic layer etching Molecular.pdf
fig_7
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FIG. 8. Etch per cycle (EPC) in units of nm/cycle for experiments (black squares) and MD simulations (red triangles) as a function of $\mathsf{Ar}^+$ energy. Error bars represent $95\%$ confidence intervals.
sci_imageminer__atomic_layer_etching__simulation_usecase__6__fig_8
atomic-layer-etching/simulation-usecase/6/fig_8
train
materials_science
atomic_layer_etching
null
simulation
[ { "panel_id": "a", "label": "multiple scatter plot" } ]
[ { "panel_id": "a", "summary": "The scatter plot compares the EPC (etching per cycle) values measured experimentally and via MD simulations across a range of ion energies. Both datasets exhibit a positive correlation between ion energy and EPC, indicating that higher ion energies lead to more effective etchi...
[ { "panel_id": "a", "data": "| Ion Energy (eV) | EPC (Experiments, nm/cycle) | EPC (MD Simulations, nm/cycle) |\n|-----------------|-----------------------------|---------------------------------|\n| 0 | 0.0 | 0.0 |\n| 25 | 0.3 ...
[ { "panel_id": "a", "question_type": "Comparative/Trend", "question": "How do EPC values from experiments compare with MD simulatuons across increasing ion energies?", "answer_type": "Paragraph", "answer": "Both experimental and simulation results show increasing EPC with rising ion energy, indic...
[ { "panel_id": "a", "x": 0, "y": 0, "width": 541, "height": 406 } ]
{ "publication_title": "Dynamics of plasma atomic layer etching: Molecular dynamics simulations and optical emission spectroscopy", "authors": "Special Collection: Atomic Layer Etching (ALE)", "doi": "10.1116/S00003011.1", "doi_candidates": [ "10.1116/S00003011.1", "10.1116/s0003011", "10.1116/6.000...
{ "extraction_method": "MinerU", "annotation_source": "Sci-ImageMiner per-image JSON", "classification_source": "repository_annotation_json", "content_source": "repository_content_json", "doi_extraction_method": "page0_regex", "source_image_path": "train/atomic-layer-etching/simulation-usecase/6/images/fig_...
train/atomic-layer-etching/simulation-usecase/6/images/fig_8.jpg
train/atomic-layer-etching/simulation-usecase/6/images/fig_8.json
train/atomic-layer-etching/simulation-usecase/6/content.json
Dynamics of plasma atomic layer etching: Molecular dynamics simulations and optical emission spectroscopy
Special Collection: Atomic Layer Etching (ALE)
10.1116/S00003011.1
https://doi.org/10.1116/S00003011.1
2,023
Dynamics of plasma atomic layer etching Molecular.pdf
fig_8
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FIG. 9. OES signals for atomic Si (middle line), SiCl (top line), and $\mathrm{SiCl_2}$ (bottom line) for $80\mathrm{eVAr^{+}}$ Results are shown for two ALE cycles. The relative intensities of the emission intensity have been adjusted for clarity and do not correspond to densities, in general. The signal for SiCl ...
sci_imageminer__atomic_layer_etching__simulation_usecase__6__fig_9
atomic-layer-etching/simulation-usecase/6/fig_9
train
materials_science
atomic_layer_etching
null
simulation
[ { "panel_id": "a", "label": "multi spectra chart" } ]
[ { "panel_id": "a", "summary": "This line chart displays time-resolved product formation for three species ,Si, SiCl, and SiCl₂, during repeated etching cycles, each consisting of four steps. The signal intensities sharply increase during Step 1 (etchant exposure) and then decay across subsequent steps. SiCl...
[ { "panel_id": "a", "data": "| Time (s) | Si (arb. units) | SiCl (arb. units) | SiCl₂ (arb. units) |\n|----------|------------------|-------------------|---------------------|\n| 0 | 0 | 0 | 0 |\n| 1 | 150000 | 200000 | 25000...
[ { "panel_id": "a", "question_type": "Comparative/Trend", "question": "How do the intensities of Si, SiCl, and SiCl₂ evolve over time, and what trend is observed across successive cycles?", "answer_type": "Paragraph", "answer": "Across both etching cycles, SiCl₂ exhibits the highest product count...
[ { "panel_id": "a", "x": 0, "y": 0, "width": 675, "height": 466 } ]
{ "publication_title": "Dynamics of plasma atomic layer etching: Molecular dynamics simulations and optical emission spectroscopy", "authors": "Special Collection: Atomic Layer Etching (ALE)", "doi": "10.1116/S00003011.1", "doi_candidates": [ "10.1116/S00003011.1", "10.1116/s0003011", "10.1116/6.000...
{ "extraction_method": "MinerU", "annotation_source": "Sci-ImageMiner per-image JSON", "classification_source": "repository_annotation_json", "content_source": "repository_content_json", "doi_extraction_method": "page0_regex", "source_image_path": "train/atomic-layer-etching/simulation-usecase/6/images/fig_...
train/atomic-layer-etching/simulation-usecase/6/images/fig_9.jpg
train/atomic-layer-etching/simulation-usecase/6/images/fig_9.json
train/atomic-layer-etching/simulation-usecase/6/content.json
Dynamics of plasma atomic layer etching: Molecular dynamics simulations and optical emission spectroscopy
Special Collection: Atomic Layer Etching (ALE)
10.1116/S00003011.1
https://doi.org/10.1116/S00003011.1
2,023
Dynamics of plasma atomic layer etching Molecular.pdf
fig_9
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FIG. 1. (a) Simplified MicroLED structure where surface damage increasingly limits the external quantum efficiency as devices scale down. (b) The general structure of a GaN MISHEMT device showing the recess into the GaN layer. Etching of the recess using reactive ion etching can lead to a rough interface, degrading the...
sci_imageminer__atomic_layer_etching__simulation_usecase__8__fig_1
atomic-layer-etching/simulation-usecase/8/fig_1
train
materials_science
atomic_layer_etching
null
simulation
[ { "panel_id": "a", "label": "device structure diagram" }, { "panel_id": "b", "label": "device structure diagram" } ]
[ { "panel_id": "a", "summary": "A cross-sectional view of a multi-quantum well semiconductor structure, including etch damage due to ion etching." }, { "panel_id": "b", "summary": "A cross-sectional view of a GaN MISHEMT structure, including etch damage due to ion etching." } ]
[ { "panel_id": "a", "data": "" }, { "panel_id": "b", "data": "" } ]
[ { "panel_id": "a", "question_type": "Application/Performance", "question": "With what material is the quantum well doped?", "answer_type": "Factoid", "answer": "The well is doped with indium." }, { "panel_id": "a", "question_type": "Process-Oriented", "question": "How can the sid...
[ { "panel_id": "a", "x": 2, "y": 2, "width": 669, "height": 396 }, { "panel_id": "b", "x": 0, "y": 436, "width": 671, "height": 368 } ]
{ "publication_title": "Isotropic atomic layer etching of GaN using $\\mathsf{SF}_6$ plasma and $\\mathsf{Al(CH_3)_3}$", "authors": "Nicholas J. Chittock $\\oplus$ ; Yi Shu; Simon D. Elliott $\\oplus$ ; Harm C. M. Knoops $\\oplus$ ; W. M. M. (Erwin). Kessels $\\oplus$ ; Adriaan J. M. Mackus $\\oplus$", ...
{ "extraction_method": "MinerU", "annotation_source": "Sci-ImageMiner per-image JSON", "classification_source": "repository_annotation_json", "content_source": "repository_content_json", "doi_extraction_method": "page0_regex", "source_image_path": "train/atomic-layer-etching/simulation-usecase/8/images/fig_...
train/atomic-layer-etching/simulation-usecase/8/images/fig_1.jpg
train/atomic-layer-etching/simulation-usecase/8/images/fig_1.json
train/atomic-layer-etching/simulation-usecase/8/content.json
Isotropic atomic layer etching of GaN using $\mathsf{SF}_6$ plasma and $\mathsf{Al(CH_3)_3}$
Nicholas J. Chittock $\oplus$ ; Yi Shu; Simon D. Elliott $\oplus$ ; Harm C. M. Knoops $\oplus$ ; W. M. M. (Erwin). Kessels $\oplus$ ; Adriaan J. M. Mackus $\oplus$
10.1063/510158129
https://doi.org/10.1063/510158129
2,023
Isotropic atomic layer etching of GaN using SF6 plasma and AI(CH3)3.pdf
fig_1
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1.0.0
FIG. 10. Atomic percentages of F, O, S, and C at the etched surface from XPS as a function of ALE cycles at $300^{\circ}\mathrm{C}$ . Lines are a guide to the eye.
sci_imageminer__atomic_layer_etching__simulation_usecase__8__fig_10
atomic-layer-etching/simulation-usecase/8/fig_10
train
materials_science
atomic_layer_etching
null
simulation
[ { "panel_id": "a", "label": "multiple scatter plot" } ]
[ { "panel_id": "a", "summary": "The chart shows the atomic percent of O1s, C1s, F1s, and S2p elements as a function of ALE cycles." } ]
[ { "panel_id": "a", "data": "| ALE cycles | O1s | C1s | F1s | S2p |\n|---|---|---|---|---|\n| 0 | 15 | 14 | 2 | 0 |\n| 10 | 10 | 6 | 6 | 2 |\n| 20 | 10 | 6 | 6 | 2 |\n| 30 | 9 | 6 | 6 | 2 |\n| 50 | 9 | 6 | 6 | 2 |\n| 70 | 8 | 6 | 6 | 2 |" } ]
[ { "panel_id": "a", "question_type": "Structure-Property", "question": "What elements are removed with this ALE process?", "answer_type": "Factoid", "answer": "The ALE process removes oxygen and carbon species." }, { "panel_id": "a", "question_type": "Application/Performance", "qu...
[ { "panel_id": "a", "x": 3, "y": 2, "width": 666, "height": 517 } ]
{ "publication_title": "Isotropic atomic layer etching of GaN using $\\mathsf{SF}_6$ plasma and $\\mathsf{Al(CH_3)_3}$", "authors": "Nicholas J. Chittock $\\oplus$ ; Yi Shu; Simon D. Elliott $\\oplus$ ; Harm C. M. Knoops $\\oplus$ ; W. M. M. (Erwin). Kessels $\\oplus$ ; Adriaan J. M. Mackus $\\oplus$", ...
{ "extraction_method": "MinerU", "annotation_source": "Sci-ImageMiner per-image JSON", "classification_source": "repository_annotation_json", "content_source": "repository_content_json", "doi_extraction_method": "page0_regex", "source_image_path": "train/atomic-layer-etching/simulation-usecase/8/images/fig_...
train/atomic-layer-etching/simulation-usecase/8/images/fig_10.jpg
train/atomic-layer-etching/simulation-usecase/8/images/fig_10.json
train/atomic-layer-etching/simulation-usecase/8/content.json
Isotropic atomic layer etching of GaN using $\mathsf{SF}_6$ plasma and $\mathsf{Al(CH_3)_3}$
Nicholas J. Chittock $\oplus$ ; Yi Shu; Simon D. Elliott $\oplus$ ; Harm C. M. Knoops $\oplus$ ; W. M. M. (Erwin). Kessels $\oplus$ ; Adriaan J. M. Mackus $\oplus$
10.1063/510158129
https://doi.org/10.1063/510158129
2,023
Isotropic atomic layer etching of GaN using SF6 plasma and AI(CH3)3.pdf
fig_10
672
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CC BY 4.0
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non_commercial_research_use_only
1.0.0
FIG. 11. Al2p XPS peak area and peak binding energy after 30 ALE cycles as a function of table temperature. The binding energies of $\mathrm{AlF}_3$ and $\mathrm{Al}_2\mathrm{O}_3$ have been included as dashed lines to show the transition between the two binding environments. The insets show the fitted Al2p XPS spe...
sci_imageminer__atomic_layer_etching__simulation_usecase__8__fig_11
atomic-layer-etching/simulation-usecase/8/fig_11
train
materials_science
atomic_layer_etching
null
simulation
[ { "panel_id": "a", "label": "multi-axis chart" }, { "panel_id": "b", "label": "spectra chart" } ]
[ { "panel_id": "a", "summary": "The chart shows the relationship between the table temperature and the Al2p peak area and peak binding energy of AlF3 and Al2O3." }, { "panel_id": "b", "summary": "The inset spectra chart displays the intensity of Al2p peaks at different binding energies." } ]
[ { "panel_id": "a", "data": "| Table temperature°C | Al2p peak area (CPS eV) | Peak binding energy (eV) |\n|---|---|---|\n| 100 | 17000 | 76.0 |\n| 125 | 17000 | 76.0 |\n| 150 | 15000 | 76.0 |\n| 175 | 5000 | 75.7|\n| 200 | 2000 | 74.7 |\n| 225 | 2000 | 74.5 |\n| 250 | 2000 | 74.7 |\n| 275 | 2000 | 74.5 |\n|...
[ { "panel_id": "a", "question_type": "Process-Oriented", "question": "What could be the reason for the shift from AlF3 to Al2O3 upon increasing the table temperature?", "answer_type": "Paragraph", "answer": "A reason could be that fluorine species get more volatile at higher temperatures, meaning...
[ { "panel_id": "a", "x": 0, "y": 2, "width": 669, "height": 515 }, { "panel_id": "b", "x": 246, "y": 123, "width": 162, "height": 160 } ]
{ "publication_title": "Isotropic atomic layer etching of GaN using $\\mathsf{SF}_6$ plasma and $\\mathsf{Al(CH_3)_3}$", "authors": "Nicholas J. Chittock $\\oplus$ ; Yi Shu; Simon D. Elliott $\\oplus$ ; Harm C. M. Knoops $\\oplus$ ; W. M. M. (Erwin). Kessels $\\oplus$ ; Adriaan J. M. Mackus $\\oplus$", ...
{ "extraction_method": "MinerU", "annotation_source": "Sci-ImageMiner per-image JSON", "classification_source": "repository_annotation_json", "content_source": "repository_content_json", "doi_extraction_method": "page0_regex", "source_image_path": "train/atomic-layer-etching/simulation-usecase/8/images/fig_...
train/atomic-layer-etching/simulation-usecase/8/images/fig_11.jpg
train/atomic-layer-etching/simulation-usecase/8/images/fig_11.json
train/atomic-layer-etching/simulation-usecase/8/content.json
Isotropic atomic layer etching of GaN using $\mathsf{SF}_6$ plasma and $\mathsf{Al(CH_3)_3}$
Nicholas J. Chittock $\oplus$ ; Yi Shu; Simon D. Elliott $\oplus$ ; Harm C. M. Knoops $\oplus$ ; W. M. M. (Erwin). Kessels $\oplus$ ; Adriaan J. M. Mackus $\oplus$
10.1063/510158129
https://doi.org/10.1063/510158129
2,023
Isotropic atomic layer etching of GaN using SF6 plasma and AI(CH3)3.pdf
fig_11
675
523
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CC BY 4.0
source_publisher_rights_reserved
non_commercial_research_use_only
1.0.0
FIG. 2. Schematic of the standard ALE process used in this work. Half-cycle A is a 10 s Ar/SF6 plasma. Half-cycle B is a TMA dose and hold, repeated four times per cycle. Each half-cycle ends with a purge before the next half-cycle. Pressure is maintained by an automated pressure controller and the inductively coupled ...
sci_imageminer__atomic_layer_etching__simulation_usecase__8__fig_2
atomic-layer-etching/simulation-usecase/8/fig_2
train
materials_science
atomic_layer_etching
null
simulation
[ { "panel_id": "a", "label": "process timing diagram" } ]
[ { "panel_id": "a", "summary": "A process flow diagram illustrating the sequence of operations and gas flow rates during two half-cycles (A and B) in a plasma process." } ]
[ { "panel_id": "a", "data": "| Time (s)| Ar (sccm)| SF6 (sccm)|TMA (pulses)|Pressure (mTorr)|ICP(W)|\n|---|---|---|---|---|---|\n|0-5|150|50|0|100|0|\n|5-15|150|50|0|100|100|\n|15-25|300|0|0|-|0|\n|25-33.4|10|0|4|150|0|\n|33.4-58.4|300|0|0|-|0|" } ]
[ { "panel_id": "a", "question_type": "Process-Oriented", "question": "What processing gas is used in this reactor?", "answer_type": "Paragraph", "answer": "Argon is used as processing gas, this is usually done as it is inert." }, { "panel_id": "a", "question_type": "Process-Oriented",...
[ { "panel_id": "a", "x": 0, "y": 1, "width": 1181, "height": 376 } ]
{ "publication_title": "Isotropic atomic layer etching of GaN using $\\mathsf{SF}_6$ plasma and $\\mathsf{Al(CH_3)_3}$", "authors": "Nicholas J. Chittock $\\oplus$ ; Yi Shu; Simon D. Elliott $\\oplus$ ; Harm C. M. Knoops $\\oplus$ ; W. M. M. (Erwin). Kessels $\\oplus$ ; Adriaan J. M. Mackus $\\oplus$", ...
{ "extraction_method": "MinerU", "annotation_source": "Sci-ImageMiner per-image JSON", "classification_source": "repository_annotation_json", "content_source": "repository_content_json", "doi_extraction_method": "page0_regex", "source_image_path": "train/atomic-layer-etching/simulation-usecase/8/images/fig_...
train/atomic-layer-etching/simulation-usecase/8/images/fig_2.jpg
train/atomic-layer-etching/simulation-usecase/8/images/fig_2.json
train/atomic-layer-etching/simulation-usecase/8/content.json
Isotropic atomic layer etching of GaN using $\mathsf{SF}_6$ plasma and $\mathsf{Al(CH_3)_3}$
Nicholas J. Chittock $\oplus$ ; Yi Shu; Simon D. Elliott $\oplus$ ; Harm C. M. Knoops $\oplus$ ; W. M. M. (Erwin). Kessels $\oplus$ ; Adriaan J. M. Mackus $\oplus$
10.1063/510158129
https://doi.org/10.1063/510158129
2,023
Isotropic atomic layer etching of GaN using SF6 plasma and AI(CH3)3.pdf
fig_2
1,180
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CC BY 4.0
source_publisher_rights_reserved
non_commercial_research_use_only
1.0.0
FIG. 3. (a) Contributions of Ga-O and Ga-N to the Ga3d peak area plotted as a function of sputter depth. The vertical dashed line indicates the spectra shown in (b). (b) The Ga3d signal after $20\mathrm{s}$ of sputtering, highlighting the positions of the Ga-O and the Ga-N peaks at $20.5$ and $19.3\mathrm{eV}$ , r...
sci_imageminer__atomic_layer_etching__simulation_usecase__8__fig_3
atomic-layer-etching/simulation-usecase/8/fig_3
train
materials_science
atomic_layer_etching
null
simulation
[ { "panel_id": "a", "label": "multiple scatter plot" }, { "panel_id": "b", "label": "multi spectra chart" } ]
[ { "panel_id": "a", "summary": "The line chart shows the peak area of XPS signals for Ga-N and Ga-O as a function of sputter depth." }, { "panel_id": "b", "summary": "The spectrum displays the XPS counts at various binding energies for Ga-N and Ga-O." } ]
[ { "panel_id": "a", "data": "| Sputter depth (nm)| Peak area (CPS eV) Ga-O| Peak area (CPS eV) Ga-N|\n|---|---|---|\n| 0 | 4000 |0|\n|5|1300|4500|\n|10|1000|5000|\n|15|1000|5000|\n|20|1000|5000|\n|25|0|5700|\n|30|0|6000|\n|35|0|5700|\n|40|0|500|" }, { "panel_id": "b", "data": "| Binding energy (e...
[ { "panel_id": "a", "question_type": "Comparative/Trend", "question": "From what depth of sputtering is there no Ga-O in the film?", "answer_type": "Factoid", "answer": "From 25 nm and deeper." }, { "panel_id": "a", "question_type": "Process-Oriented", "question": "Can the type of...
[ { "panel_id": "a", "x": 0, "y": 12, "width": 346, "height": 427 }, { "panel_id": "b", "x": 384, "y": 12, "width": 282, "height": 427 } ]
{ "publication_title": "Isotropic atomic layer etching of GaN using $\\mathsf{SF}_6$ plasma and $\\mathsf{Al(CH_3)_3}$", "authors": "Nicholas J. Chittock $\\oplus$ ; Yi Shu; Simon D. Elliott $\\oplus$ ; Harm C. M. Knoops $\\oplus$ ; W. M. M. (Erwin). Kessels $\\oplus$ ; Adriaan J. M. Mackus $\\oplus$", ...
{ "extraction_method": "MinerU", "annotation_source": "Sci-ImageMiner per-image JSON", "classification_source": "repository_annotation_json", "content_source": "repository_content_json", "doi_extraction_method": "page0_regex", "source_image_path": "train/atomic-layer-etching/simulation-usecase/8/images/fig_...
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train/atomic-layer-etching/simulation-usecase/8/images/fig_3.json
train/atomic-layer-etching/simulation-usecase/8/content.json
Isotropic atomic layer etching of GaN using $\mathsf{SF}_6$ plasma and $\mathsf{Al(CH_3)_3}$
Nicholas J. Chittock $\oplus$ ; Yi Shu; Simon D. Elliott $\oplus$ ; Harm C. M. Knoops $\oplus$ ; W. M. M. (Erwin). Kessels $\oplus$ ; Adriaan J. M. Mackus $\oplus$
10.1063/510158129
https://doi.org/10.1063/510158129
2,023
Isotropic atomic layer etching of GaN using SF6 plasma and AI(CH3)3.pdf
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FIG. 4. Gibbs free energy change $(\Delta \mathbb{G})$ as a function of temperature for the fluorination half-cycle considering both the conversion (blue) and chemical vapor etching (red) reactions. Solid lines indicate plasma fluorination reactions (F radicals), while the thermal fluorination reactions (HF) are indi...
sci_imageminer__atomic_layer_etching__simulation_usecase__8__fig_4
atomic-layer-etching/simulation-usecase/8/fig_4
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materials_science
atomic_layer_etching
null
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[ { "panel_id": "a", "label": "multiple line chart" } ]
[ { "panel_id": "a", "summary": "The chart illustrates the change in Gibbs free energy (ΔG) per unit GaN with respect to temperature for various etching methods." } ]
[ { "panel_id": "a", "data": "| Temperature (°C) | ΔG (eV/GaN) HF CVE |ΔG (eV/GaN) HF conversion |ΔG (eV/GaN) TMA ligand-exchange |ΔG (eV/GaN) F radical CVE |ΔG (eV/GaN) F radical conversion |\n|---|---|---|---|---|---|\n|-200 | 0 |-3|-0.5|-18.5|-21|\n|-100 | 0 |-2|-1|-18|-20|\n|0 | 0.5 |-2|-1.5|-16|-19|\n|10...
[ { "panel_id": "a", "question_type": "Process-Oriented", "question": "What is more energetically favorable with resect to temperature, the use of HF or the use of SF6?", "answer_type": "Paragraph", "answer": "The use of F radicals in a plasma as this lowers the gibbs energy the most." }, { ...
[ { "panel_id": "a", "x": 5, "y": 3, "width": 650, "height": 532 } ]
{ "publication_title": "Isotropic atomic layer etching of GaN using $\\mathsf{SF}_6$ plasma and $\\mathsf{Al(CH_3)_3}$", "authors": "Nicholas J. Chittock $\\oplus$ ; Yi Shu; Simon D. Elliott $\\oplus$ ; Harm C. M. Knoops $\\oplus$ ; W. M. M. (Erwin). Kessels $\\oplus$ ; Adriaan J. M. Mackus $\\oplus$", ...
{ "extraction_method": "MinerU", "annotation_source": "Sci-ImageMiner per-image JSON", "classification_source": "repository_annotation_json", "content_source": "repository_content_json", "doi_extraction_method": "page0_regex", "source_image_path": "train/atomic-layer-etching/simulation-usecase/8/images/fig_...
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train/atomic-layer-etching/simulation-usecase/8/images/fig_4.json
train/atomic-layer-etching/simulation-usecase/8/content.json
Isotropic atomic layer etching of GaN using $\mathsf{SF}_6$ plasma and $\mathsf{Al(CH_3)_3}$
Nicholas J. Chittock $\oplus$ ; Yi Shu; Simon D. Elliott $\oplus$ ; Harm C. M. Knoops $\oplus$ ; W. M. M. (Erwin). Kessels $\oplus$ ; Adriaan J. M. Mackus $\oplus$
10.1063/510158129
https://doi.org/10.1063/510158129
2,023
Isotropic atomic layer etching of GaN using SF6 plasma and AI(CH3)3.pdf
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FIG. 5. Saturation curves at 150 and $300^{\circ}\mathrm{C}$ for (a) $\mathrm{SF}_6$ plasma exposure using $10\times 100\mathrm{ms}$ TMA exposures and (b) varied number of $100\mathrm{ms}$ TMA pulses with a $10\mathrm{s}$ $\mathrm{SF}_6$ plasma step, determined over 30 ALE cycles. Lines are guides for the eye...
sci_imageminer__atomic_layer_etching__simulation_usecase__8__fig_5
atomic-layer-etching/simulation-usecase/8/fig_5
train
materials_science
atomic_layer_etching
null
simulation
[ { "panel_id": "a", "label": "multiple scatter plot" }, { "panel_id": "b", "label": "multiple scatter plot" } ]
[ { "panel_id": "a", "summary": "The line chart shows the relationship between SF₆ plasma time and EPC (nm/cycle) at two temperatures, 300°C and 150°C." }, { "panel_id": "b", "summary": "The line chart illustrates the relationship between TMA pulses and EPC (nm/cycle) at two temperatures, 300°C an...
[ { "panel_id": "a", "data": "| SF₆ plasma time (s) | EPC (nm/cycle) 300 degrees |EPC (nm/cycle) 150 degrees |\n|---|---|---|\n| 0 | 0.0 |0.0|\n| 5 | 0.37 |0.27|\n| 10 | 0.4 |0.3|\n| 15 | 0.41 |0.31|\n| 30 | 0.41 |0.35|" }, { "panel_id": "b", "data": "| TMA pulses | EPC (nm/cycle) 300 degrees |EPC...
[ { "panel_id": "a", "question_type": "Process-Oriented", "question": "Why is the saturated EPC higher for higher temperatures?", "answer_type": "Paragraph", "answer": "It could be that the penetration depth of the radical species increases for increasing temperature." }, { "panel_id": "a"...
[ { "panel_id": "a", "x": 1, "y": 4, "width": 371, "height": 491 }, { "panel_id": "b", "x": 387, "y": 4, "width": 284, "height": 491 } ]
{ "publication_title": "Isotropic atomic layer etching of GaN using $\\mathsf{SF}_6$ plasma and $\\mathsf{Al(CH_3)_3}$", "authors": "Nicholas J. Chittock $\\oplus$ ; Yi Shu; Simon D. Elliott $\\oplus$ ; Harm C. M. Knoops $\\oplus$ ; W. M. M. (Erwin). Kessels $\\oplus$ ; Adriaan J. M. Mackus $\\oplus$", ...
{ "extraction_method": "MinerU", "annotation_source": "Sci-ImageMiner per-image JSON", "classification_source": "repository_annotation_json", "content_source": "repository_content_json", "doi_extraction_method": "page0_regex", "source_image_path": "train/atomic-layer-etching/simulation-usecase/8/images/fig_...
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train/atomic-layer-etching/simulation-usecase/8/images/fig_5.json
train/atomic-layer-etching/simulation-usecase/8/content.json
Isotropic atomic layer etching of GaN using $\mathsf{SF}_6$ plasma and $\mathsf{Al(CH_3)_3}$
Nicholas J. Chittock $\oplus$ ; Yi Shu; Simon D. Elliott $\oplus$ ; Harm C. M. Knoops $\oplus$ ; W. M. M. (Erwin). Kessels $\oplus$ ; Adriaan J. M. Mackus $\oplus$
10.1063/510158129
https://doi.org/10.1063/510158129
2,023
Isotropic atomic layer etching of GaN using SF6 plasma and AI(CH3)3.pdf
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FIG. 6. Synergy plot for GaN using $\mathrm{SF}_6$ plasma and TMA at $300^{\circ}\mathrm{C}$ . The first 25 pulses only involve dosing $\mathrm{SF}_6$ plasma, the next 25 pulses only TMA, and the last 75 cycles are full ALE cycles with both $\mathrm{SF}_6$ plasma and TMA dosed. The inset shows the transition bet...
sci_imageminer__atomic_layer_etching__simulation_usecase__8__fig_6
atomic-layer-etching/simulation-usecase/8/fig_6
train
materials_science
atomic_layer_etching
null
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[ { "panel_id": "a", "label": "scatter plot" } ]
[ { "panel_id": "a", "summary": "The line chart illustrates the relationship between film thickness and pulses/cycles, showing a decreasing trend if both reactants are dosed." } ]
[ { "panel_id": "a", "data": "| Pulses/Cycles | Film thickness (nm) |\n|---|---|\n| 0 | 43 |\n| 25 | 43 |\n| 50 | 42 |\n| 75 | 33 |\n| 100 | 25 |\n| 125 | 18 |" } ]
[ { "panel_id": "a", "question_type": "Process-Oriented", "question": "Based on the first 50 pulses/cycles, what is the etch per cycle and where can this be found?", "answer_type": "Paragraph", "answer": "At 25 pulses/cycles the SF6 plasma dosing is switched with TMA dosing, here a drop of 0.33 nm...
[ { "panel_id": "a", "x": 2, "y": 1, "width": 669, "height": 510 } ]
{ "publication_title": "Isotropic atomic layer etching of GaN using $\\mathsf{SF}_6$ plasma and $\\mathsf{Al(CH_3)_3}$", "authors": "Nicholas J. Chittock $\\oplus$ ; Yi Shu; Simon D. Elliott $\\oplus$ ; Harm C. M. Knoops $\\oplus$ ; W. M. M. (Erwin). Kessels $\\oplus$ ; Adriaan J. M. Mackus $\\oplus$", ...
{ "extraction_method": "MinerU", "annotation_source": "Sci-ImageMiner per-image JSON", "classification_source": "repository_annotation_json", "content_source": "repository_content_json", "doi_extraction_method": "page0_regex", "source_image_path": "train/atomic-layer-etching/simulation-usecase/8/images/fig_...
train/atomic-layer-etching/simulation-usecase/8/images/fig_6.jpg
train/atomic-layer-etching/simulation-usecase/8/images/fig_6.json
train/atomic-layer-etching/simulation-usecase/8/content.json
Isotropic atomic layer etching of GaN using $\mathsf{SF}_6$ plasma and $\mathsf{Al(CH_3)_3}$
Nicholas J. Chittock $\oplus$ ; Yi Shu; Simon D. Elliott $\oplus$ ; Harm C. M. Knoops $\oplus$ ; W. M. M. (Erwin). Kessels $\oplus$ ; Adriaan J. M. Mackus $\oplus$
10.1063/510158129
https://doi.org/10.1063/510158129
2,023
Isotropic atomic layer etching of GaN using SF6 plasma and AI(CH3)3.pdf
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FIG. 7. GaN EPC as a function of table temperature. Data for $\mathrm{Al}_2\mathrm{O}_3$ ALE using the same $\mathrm{SF}_6$ plasma/TMA chemistry are shown from our previous work. Thermal GaN ALE with $\mathrm{XeF}_2 / \mathrm{BCl}_3$ is also included in the plot. Lines are guides to the eye.
sci_imageminer__atomic_layer_etching__simulation_usecase__8__fig_7
atomic-layer-etching/simulation-usecase/8/fig_7
train
materials_science
atomic_layer_etching
null
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[ { "panel_id": "a", "label": "multiple scatter plot" } ]
[ { "panel_id": "a", "summary": "The chart shows the EPC (nm/cycle) of Plasma ALE GaN, Plasma ALE Al₂O₃, and Thermal ALE GaN at various temperatures. The data points are connected by lines, indicating trends over temperature." } ]
[ { "panel_id": "a", "data": "| Temperature (°C) | Plasma ALE GaN | Plasma ALE Al₂O₃ | Thermal ALE GaN |\n|-----------------|----------------|------------------|----------------|\n| 100 | 0.0 | 0.0 | 0.0 |\n| 150 | 0.2 | 0.0 | 0....
[ { "panel_id": "a", "question_type": "Process-Oriented", "question": "Is there a selectivity window with the SF6/TMA chemistry?", "answer_type": "Paragraph", "answer": "Yes there is a selectivity window between 100 and 175 degrees celcius, so GaN can be etched selectively wrt Al2O3." }, { ...
[ { "panel_id": "a", "x": 4, "y": 4, "width": 659, "height": 547 } ]
{ "publication_title": "Isotropic atomic layer etching of GaN using $\\mathsf{SF}_6$ plasma and $\\mathsf{Al(CH_3)_3}$", "authors": "Nicholas J. Chittock $\\oplus$ ; Yi Shu; Simon D. Elliott $\\oplus$ ; Harm C. M. Knoops $\\oplus$ ; W. M. M. (Erwin). Kessels $\\oplus$ ; Adriaan J. M. Mackus $\\oplus$", ...
{ "extraction_method": "MinerU", "annotation_source": "Sci-ImageMiner per-image JSON", "classification_source": "repository_annotation_json", "content_source": "repository_content_json", "doi_extraction_method": "page0_regex", "source_image_path": "train/atomic-layer-etching/simulation-usecase/8/images/fig_...
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train/atomic-layer-etching/simulation-usecase/8/images/fig_7.json
train/atomic-layer-etching/simulation-usecase/8/content.json
Isotropic atomic layer etching of GaN using $\mathsf{SF}_6$ plasma and $\mathsf{Al(CH_3)_3}$
Nicholas J. Chittock $\oplus$ ; Yi Shu; Simon D. Elliott $\oplus$ ; Harm C. M. Knoops $\oplus$ ; W. M. M. (Erwin). Kessels $\oplus$ ; Adriaan J. M. Mackus $\oplus$
10.1063/510158129
https://doi.org/10.1063/510158129
2,023
Isotropic atomic layer etching of GaN using SF6 plasma and AI(CH3)3.pdf
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FIG. 8. AFM height maps for (a) the as-deposited $43 \text{nm}$ thick GaN film and (b) after $25 \text{nm}$ ALE at $300^{\circ} \text{C}$ using the standard recipe shown in Fig. 2.
sci_imageminer__atomic_layer_etching__simulation_usecase__8__fig_8
atomic-layer-etching/simulation-usecase/8/fig_8
train
materials_science
atomic_layer_etching
null
simulation
[ { "panel_id": "a", "label": "heatmap" }, { "panel_id": "b", "label": "heatmap" } ]
[ { "panel_id": "a", "summary": "The figure shows an AFM image with a color gradient indicating height in nanometers. The x-axis represents the horizontal position in micrometers, and the y-axis represents the vertical position in micrometers." }, { "panel_id": "b", "summary": "The figure shows an...
[ { "panel_id": "a", "data": "" }, { "panel_id": "b", "data": "" } ]
[ { "panel_id": "a", "question_type": "Comparative/Trend", "question": "What is the biggest height difference on the image and how can they be called?", "answer_type": "Paragraph", "answer": "The biggest height difference is around 13 nm, these can be called pinholes." }, { "panel_id": "a"...
[ { "panel_id": "a", "x": 3, "y": 3, "width": 703, "height": 552 }, { "panel_id": "b", "x": 707, "y": 3, "width": 696, "height": 555 } ]
{ "publication_title": "Isotropic atomic layer etching of GaN using $\\mathsf{SF}_6$ plasma and $\\mathsf{Al(CH_3)_3}$", "authors": "Nicholas J. Chittock $\\oplus$ ; Yi Shu; Simon D. Elliott $\\oplus$ ; Harm C. M. Knoops $\\oplus$ ; W. M. M. (Erwin). Kessels $\\oplus$ ; Adriaan J. M. Mackus $\\oplus$", ...
{ "extraction_method": "MinerU", "annotation_source": "Sci-ImageMiner per-image JSON", "classification_source": "repository_annotation_json", "content_source": "repository_content_json", "doi_extraction_method": "page0_regex", "source_image_path": "train/atomic-layer-etching/simulation-usecase/8/images/fig_...
train/atomic-layer-etching/simulation-usecase/8/images/fig_8.jpg
train/atomic-layer-etching/simulation-usecase/8/images/fig_8.json
train/atomic-layer-etching/simulation-usecase/8/content.json
Isotropic atomic layer etching of GaN using $\mathsf{SF}_6$ plasma and $\mathsf{Al(CH_3)_3}$
Nicholas J. Chittock $\oplus$ ; Yi Shu; Simon D. Elliott $\oplus$ ; Harm C. M. Knoops $\oplus$ ; W. M. M. (Erwin). Kessels $\oplus$ ; Adriaan J. M. Mackus $\oplus$
10.1063/510158129
https://doi.org/10.1063/510158129
2,023
Isotropic atomic layer etching of GaN using SF6 plasma and AI(CH3)3.pdf
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FIG. 9. RMS roughness as a function of etched thickness, plotted alongside the fitted change in RMS roughness as obtained using the curvature-dependent model from Ref. 85.
sci_imageminer__atomic_layer_etching__simulation_usecase__8__fig_9
atomic-layer-etching/simulation-usecase/8/fig_9
train
materials_science
atomic_layer_etching
null
simulation
[ { "panel_id": "a", "label": "scatter plot" } ]
[ { "panel_id": "a", "summary": "The line chart shows the relationship between etched thickness and RMS roughness, with experimental data points and a curvature-dependent model curve." } ]
[ { "panel_id": "a", "data": "| Etched thickness (nm) | RMS roughness (nm) |\n|---|---|\n| 0 | 2.65 |\n| 5 | 2.4 |\n| 10 | 2.2 |\n| 15 | 2.0 |\n| 20 | 2.0 |\n| 25 | 1.9 |" } ]
[ { "panel_id": "a", "question_type": "Process-Oriented", "question": "What could be a reason for the initial RMS of 2.65 nm?", "answer_type": "Paragraph", "answer": "It could be that there is dust incorporated in the film or the deposition method with which the GaN is made is not uniform." }, ...
[ { "panel_id": "a", "x": 3, "y": 6, "width": 666, "height": 527 } ]
{ "publication_title": "Isotropic atomic layer etching of GaN using $\\mathsf{SF}_6$ plasma and $\\mathsf{Al(CH_3)_3}$", "authors": "Nicholas J. Chittock $\\oplus$ ; Yi Shu; Simon D. Elliott $\\oplus$ ; Harm C. M. Knoops $\\oplus$ ; W. M. M. (Erwin). Kessels $\\oplus$ ; Adriaan J. M. Mackus $\\oplus$", ...
{ "extraction_method": "MinerU", "annotation_source": "Sci-ImageMiner per-image JSON", "classification_source": "repository_annotation_json", "content_source": "repository_content_json", "doi_extraction_method": "page0_regex", "source_image_path": "train/atomic-layer-etching/simulation-usecase/8/images/fig_...
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train/atomic-layer-etching/simulation-usecase/8/images/fig_9.json
train/atomic-layer-etching/simulation-usecase/8/content.json
Isotropic atomic layer etching of GaN using $\mathsf{SF}_6$ plasma and $\mathsf{Al(CH_3)_3}$
Nicholas J. Chittock $\oplus$ ; Yi Shu; Simon D. Elliott $\oplus$ ; Harm C. M. Knoops $\oplus$ ; W. M. M. (Erwin). Kessels $\oplus$ ; Adriaan J. M. Mackus $\oplus$
10.1063/510158129
https://doi.org/10.1063/510158129
2,023
Isotropic atomic layer etching of GaN using SF6 plasma and AI(CH3)3.pdf
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Fig. A1. Convergce tests for atomic layr nmber and cutoff energies for DFT calculations. (a) Variation of adsorption energy of chlorine with layer number, cutoff energies of $50 / 200\mathrm{Ry}$ were applied. (b) Variation of total system energy with cutoff energies for wave function and electron density, the cutoff...
sci_imageminer__atomic_layer_etching__simulation_usecase__9__1efb120580ad0809db6986794a53a1e9c383b07153d625e10037bb0738d83671
atomic-layer-etching/simulation-usecase/9/1efb120580ad0809db6986794a53a1e9c383b07153d625e10037bb0738d83671
train
materials_science
atomic_layer_etching
null
simulation
[ { "panel_id": "a", "label": "line chart" }, { "panel_id": "b", "label": "line chart" } ]
[ { "panel_id": "a", "summary": "The line chart shows the relationship between layer number and adsorption energy, with a decreasing trend, indicating that for a certain structure adsorption is more likely." }, { "panel_id": "b", "summary": "The line chart illustrates the decrease in total energy ...
[ { "panel_id": "a", "data": "| Layer number | Adsorption Energy (eV) |\n|---|---|\n| 4 | 4.2 |\n| 6 | 4.13 |\n| 8 | 4.12 |\n| 10 | 4.12 |\n| 12 | 4.12 |" }, { "panel_id": "b", "data": "| Cut-off energies (Ry) | Total energy (Ry) |\n|---|---|\n| 15 | -945.9 |\n| 20 | -946.1 |\n| 25 | -946.2 |\n| 3...
[ { "panel_id": "a", "question_type": "Structure-Property", "question": "What could be the reason that for increasing layer number the adsorption energy levels of?", "answer_type": "Paragraph", "answer": "It could be that from a certain thickness onwards, the substrate has no repelling influence o...
[ { "panel_id": "a", "x": 9, "y": 11, "width": 654, "height": 400 }, { "panel_id": "b", "x": 7, "y": 455, "width": 654, "height": 391 } ]
{ "publication_title": "Mechanism of photo-assisted atomic layer etching of chlorinated Si(111) surfaces: Insights from DFT/TDDFT calculations", "authors": "Peizhi Wang a, Marco Castelli a, Fengzhou Fang a,b,*", "doi": null, "doi_candidates": [], "url": null, "publication_year": null, "journal_or_venue": ...
{ "extraction_method": "MinerU", "annotation_source": "Sci-ImageMiner per-image JSON", "classification_source": "repository_annotation_json", "content_source": "repository_content_json", "doi_extraction_method": null, "source_image_path": "train/atomic-layer-etching/simulation-usecase/9/images/1efb120580ad0...
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train/atomic-layer-etching/simulation-usecase/9/content.json
Mechanism of photo-assisted atomic layer etching of chlorinated Si(111) surfaces: Insights from DFT/TDDFT calculations
Peizhi Wang a, Marco Castelli a, Fengzhou Fang a,b,*
null
null
null
Mechanism of photoassisted atomic layer etching of chlorinated Si(111) surfaces Insight.pdf
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Fig. A2. Variation of the lowest excitation energy with the number of Si atoms of the cluster, insets are the molecular structures of the associated clusters.
sci_imageminer__atomic_layer_etching__simulation_usecase__9__42b2341dcb88232a2b3d8fc38fe7c5cbc5345d5e59715edb80a39db016f6f34c
atomic-layer-etching/simulation-usecase/9/42b2341dcb88232a2b3d8fc38fe7c5cbc5345d5e59715edb80a39db016f6f34c
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materials_science
atomic_layer_etching
null
simulation
[ { "panel_id": "a", "label": "line chart" } ]
[ { "panel_id": "a", "summary": "The excitation energy of a system decreases as the number of silicon (Si) atoms increases, this is a stepwise relation as a function of the number of Si atoms." } ]
[ { "panel_id": "a", "data": "| Number of Si atoms | Excitation energy (eV) |\n|---|---|\n| 0 | - |\n| 3 | 4.1 |\n| 7 | 3.7 |\n| 11 | 3.6 |\n| 15 | 3.2 |\n| 24 | 3.2 |\n| 34 | 3.1 |" } ]
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Mechanism of photo-assisted atomic layer etching of chlorinated Si(111) surfaces: Insights from DFT/TDDFT calculations
Peizhi Wang a, Marco Castelli a, Fengzhou Fang a,b,*
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Mechanism of photoassisted atomic layer etching of chlorinated Si(111) surfaces Insight.pdf
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Fig. A3. Algorithm for the calculation of time evolution.
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Mechanism of photo-assisted atomic layer etching of chlorinated Si(111) surfaces: Insights from DFT/TDDFT calculations
Peizhi Wang a, Marco Castelli a, Fengzhou Fang a,b,*
null
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Mechanism of photoassisted atomic layer etching of chlorinated Si(111) surfaces Insight.pdf
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Fig. 1. Schematic of the photo-assistant ALE of chlorinated Si surfaces. The surface is modified by chlorine to weaken the back-bonds of target Si atomic layer; and then the modified Si layer is selectively removed/desorbed by $\mathrm{Ar^{+}}$ bombardment assisted by photo-irradiation.
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Mechanism of photo-assisted atomic layer etching of chlorinated Si(111) surfaces: Insights from DFT/TDDFT calculations
Peizhi Wang a, Marco Castelli a, Fengzhou Fang a,b,*
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Mechanism of photoassisted atomic layer etching of chlorinated Si(111) surfaces Insight.pdf
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Fig. 2. (a) Front and top views of the Si(111) - $(4\times 2)$ surface geometry, dark yellow atoms are Si-adatom and Si-restatom with a dangling bond, the red dotted lines are periodic boundary conditions (PBC). (b) The optimized geometry of chlorinated Si(111) surface, a $\mathrm{SiCl_2}$ is generated on the adato...
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Mechanism of photo-assisted atomic layer etching of chlorinated Si(111) surfaces: Insights from DFT/TDDFT calculations
Peizhi Wang a, Marco Castelli a, Fengzhou Fang a,b,*
null
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Mechanism of photoassisted atomic layer etching of chlorinated Si(111) surfaces Insight.pdf
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Fig. 3. (a) Potential energy curve for $\mathrm{SiCl_2}$ on the optimized Si(111) surface, here blue dots are the calculated data, and red line is the fitting function. $Z = 0$ represents the equilibrium position, and insets are the local views of the desorbed species. (b) Potential energy curve for the Si-adatom (...
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[ { "panel_id": "a", "data": "| Surface coordinate Z (Å) | Potential energy (eV) |\n|---|---|\n|-1 | 8 |\n|-0.5 | 1.2 |\n|0 | 0 |\n|0.5 | 0.8 |\n|1 | 1.5 |\n|1.5 | 2.2 |\n|2 | 2.4 |\n|2.5| 2.5|" }, { "panel_id": "b", "data": "| Surface coordinate Z (Å) | Potential energy (eV) |\n|---|---|\n|-1 | 8...
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Mechanism of photo-assisted atomic layer etching of chlorinated Si(111) surfaces: Insights from DFT/TDDFT calculations
Peizhi Wang a, Marco Castelli a, Fengzhou Fang a,b,*
null
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Mechanism of photoassisted atomic layer etching of chlorinated Si(111) surfaces Insight.pdf
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Fig. 4. Molecular structure of the selected cluster for TDDFT calculations. The cluster was extracted from the optimized slab (see Fig. 2(b)) and selected by convergence tests (see Fig. A2).
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Mechanism of photo-assisted atomic layer etching of chlorinated Si(111) surfaces: Insights from DFT/TDDFT calculations
Peizhi Wang a, Marco Castelli a, Fengzhou Fang a,b,*
null
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Mechanism of photoassisted atomic layer etching of chlorinated Si(111) surfaces Insight.pdf
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Fig. 5. HOMO and LOMO diagrams within the localized $\mathrm{SiCl_2}$ region, side view of Fig. 4 is selected for a better visualization.
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Mechanism of photo-assisted atomic layer etching of chlorinated Si(111) surfaces: Insights from DFT/TDDFT calculations
Peizhi Wang a, Marco Castelli a, Fengzhou Fang a,b,*
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Mechanism of photoassisted atomic layer etching of chlorinated Si(111) surfaces Insight.pdf
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Fig. 6. Hole and electron distributions related to the lowest excitation, $\mathrm{pink} =$ hole, blue $=$ electron, hole indicates the loss of electron.
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Mechanism of photo-assisted atomic layer etching of chlorinated Si(111) surfaces: Insights from DFT/TDDFT calculations
Peizhi Wang a, Marco Castelli a, Fengzhou Fang a,b,*
null
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Mechanism of photoassisted atomic layer etching of chlorinated Si(111) surfaces Insight.pdf
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Fig. 7. Schematic of the energy conversion process and snapshots of the density distribution with time evolution, the distributions on excited-state and ground-state potential energy curves are represented by solid and dashed lines, respectively. The vertical line $Z = Z_{d}$ is the defined critical value, the $\mat...
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[ { "panel_id": "a", "label": "multiple line chart" } ]
[ { "panel_id": "a", "summary": "The figure illustrates the potential energy of a system as a function of surface coordinate Z at various time points (t=0 fs, t=5 fs, t=10 fs, t=400 fs). It shows the transition between the ground state and excited state, with terms like 'Excitation', 'Quenching', and 'Evolvin...
[ { "panel_id": "a", "data": "| Surface coordinate Z (Å) | Potential energy (eV) Ground state | Potential energy (eV) Excited state | Density Ground state |Density Excited state |\n|---|---|---|---|---|\n|-0.7 | 3 |4.2|-|-|\n| 0 | 0 |3.1|Peak|Peak|\n| 1 | 1.6 |2.6|-|-|\n| 2 | 2.4 |2.5|-|-|\n| 3 | 2.5 |2.5|-|-...
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Mechanism of photo-assisted atomic layer etching of chlorinated Si(111) surfaces: Insights from DFT/TDDFT calculations
Peizhi Wang a, Marco Castelli a, Fengzhou Fang a,b,*
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Mechanism of photoassisted atomic layer etching of chlorinated Si(111) surfaces Insight.pdf
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