The first approach requires further development to improve computational speed. The second approach requires further development to automate accurate forcefield parameterization. Because of the extreme chemical diversity across thousands of MOF structures, this problem is still mostly unsolved today. For example, here we show structures in the 2014 CoRE MOF database contain more than 8 thousand different atom types based on first and second neighbors. Our results showed that atom types based on both first and second neighbors adequately capture the chemical environment, but atom types based on only first neighbors do not. For 3056 MOFs, we used density functional theory (DFT) followed by DDEC6 atomic population analysis to extract a host of important forcefield precursors: partial atomic charges; atom-in-material (AIM) C6, C8, and C10 dispersion coefficients; AIM dipole and quadrupole moments; various AIM polarizabilities; quantum Drude oscillator parameters; AIM electron cloud parameters; etc. Electrostatic parameters were validated through comparisons to the DFT-computed electrostatic potential. These forcefield precursors should find widespread applications to developing MOF force fields.A host of important performance properties for metal–organic frameworks (MOFs) and other complex materials can be calculated by modeling statistical ensembles. The principle challenge is to develop accurate and computationally efficient interaction models for these simulations. Two major approaches are (i)  6, C8, C10), polarizabilities, electron cloud parameters, radial moments, and atom types were extracted from quantum chemistry calculations for >3000 MOFs.Atom-in-material (AIM) partial charges, dipoles and quadrupoles, dispersion coefficients (C Because of their nanoporous structures, these materials attract much interest for gas storage, gas separation, catalysis, and other applications.2–6 Many thousands of MOF crystal structures have been deposited in the Cambridge Structural Database (CSD).1,7,8,115–117 Most often, these crystal structures were measured using X-ray diffraction crystallography (XRDC). Since hydrogen atoms contain no core electrons, they diffract X-rays extremely weakly.9 This makes it much harder to refine hydrogen atom positions than positions for heavier atoms.9–11 Consequently, hydrogen atom positions may be unresolved in some of the reported crystal structures. Other complications include the presence of disordered atoms, solvent molecules, and/or free ions in some of the reported MOF crystal structures.Metal–organic frameworks (MOFs) are a kind of coordination network comprised of metal atoms connected by organic linkers.et al. reported a Computation Ready Experimental (CoRE) MOF database that was constructed by first searching the CSD to identify MOFs and then partially cleaning these structures.7 The searching step was designed to identify structures containing metal atoms bonded to non-metal atoms that form 3-dimensional networks. The cleaning process was intended to fix or discard structures containing disordered atoms and partial occupancies. The cleaning process was also intended to remove solvent molecules and other small adsorbates in the MOF's pores but to retain charge-balancing ions. Finally, missing hydrogen atoms were added to some of the structures. However, this cleaning process was imperfect resulting in some structures with errors.12,13,115 This 2014 CoRE MOF database was the starting point for our study. It contains a total of 5109 structures, of which 4764 structures were modified during the cleaning process and 345 retained their original CSD structures.714,15 The 2014 CoRE database contains some structures that are MIFs.13In 2014, Chung et al. reported DDEC net atomic charges (NACs) for 2932 structures.16 In 2017, Nazarian et al. reported DFT-optimized geometries for 838 structures including 502 with computed DDEC NACs.17 Soon, a major revision of the CoRE MOF database will be published that expands the number of structures to approximately 15 thousand . Altintas et al.115 reported a comparative analysis between the 2014 CoRE MOF database and the CSD-derived MOF database of Moghadam et al.116Several follow-ups were subsequently made to the CoRE MOF database. In 2016, Nazarian 1 Owing to the large number of different metal atoms and organic linkers that could be combined in various ways, there is a nearly infinite number of potentially synthesizable MOFs.1,18–20 Computational chemistry can be an efficient way to search this vast chemical space to help identify the most promising materials to later synthesize and experimentally test.21 This will avoid unnecessary efforts to synthesize a large number of materials that do not perform well for the desired applications.Although many thousands of MOFs have been synthesized to date, this is only a tiny fraction of the number of MOFs that could potentially be made.e.g., constant NVE, NVT, NPT, μVT, μPT, NPH, etc.). Here, the properties can be roughly divided into thermodynamic properties that occur at equilibrium and dynamic properties that describe transient system response to non-equilibrium. Gas adsorption isotherms are often computed in the grand canonical (μVT) or Gibbs ensembles.22,23 Gas diffusion constants are often computed in the canonical (NVT) or microcanonical (NVE) ensembles using equilibrium molecular dynamics.24,25 System behaviors under extreme conditions, such as high pressures, low or high temperatures, applied electromagnetic fields, irradiation, high stresses, and corrosive conditions are of emerging interest.A host of important performance properties for MOFs and other complex materials can be calculated by modeling statistical ensembles  to solve the Schrodinger equation for the material's electron distribution . A somewhat larger length scale considers individual atoms interacting via a classical force field in atomistic simulations.21,28,29 Coarse-grained and continuum models treat even larger length scales.30,31When modeling statistical ensembles, an interaction model is required to compute the system's energy as a function of chemical configuration. Several different types of interaction models exist depending on the length scale at which the system is modeled. The smallest length scale considers individual electrons using an exchange–correlation theory  would describe all material types but is extremely computationally expensive. In practice, approximate exchange–correlation theories are used that describe an extremely broad range of different material types with acceptable accuracy and computational efficiency. Because exchange–correlation theories are not material specific, they should not have to be reparameterized for a new material type. In contrast, classical force fields have to be extensively parameterized for individual atoms or atom types.29,32 Because computing the system's energy is usually much faster using a classical force field than an exchange–correlation theory, classical atomistic simulations can usually be performed faster and over larger length and time scales than quantum chemistry calculations.Quantum chemistry using an exchange–correlation theory has different advantages and limitations compared to classical atomistic simulations using a force field. An exact exchange–correlation theory , London dispersion interactions, and/or short-range exchange-repulsion.44,45 When optimizing the bonded parameter values, it is orders of magnitude more efficient to fit them to atom-in-material forces across multiple geometries than to only fit them to the system's total energy across multiple geometries.46,47 Because each geometry yields many atom-in-material forces but only one total energy, fewer geometries are needed to fit the bonded parameter values to forces than to energies.Classical force fields typically contain bonded and non-bonded terms. Bonded terms describe flexibility  and have been incorporated into many flexible force fields for MOFs.48 As shown in e.g., Lennard-Jones) to two-particle interaction curves gives force fields that often overestimate liquid-phase densities.49 If the parameters of the two-body potential are adjusted to yield correct liquid-phase densities, then the two-particle interaction curve will be incorrectly described.45 This problem can be fixed by explicitly including many-body dispersion and/or many-body polarization in the force field. For example, Kiss and Baranyai showed polarizability must be included in a force field to describe liquid water accurately over a wide range of conditions.50A classical force field must contain many-body dispersion and/or many-body polarization to accurately describe system properties over a wide range of conditions.via an effective Lagrangian. CPMD improves the computational efficiency of ab initio molecular dynamics, but CPMD is limited to materials containing a band gap .52–54 VASP can perform ab initio molecular dynamics even for metals, but this requires computing self-consistent orbitals at each time step.54,55 Recently, many studies focused on first-principles derived classical force fields whose parameters are extracted from quantum chemistry calculations.22,35,40,44,45,49,56,57 Other studies parameterized force fields by fitting to experimental data36,58 or using machine learning  is a quantum chemistry method in which the wavefunction does not have to be self-consistently solved at each time step, because it evolves learning .et al.7 We attempted DFT calculations on all of the modified structures except the largest ones containing >∼1700 atoms; however, some DFT calculations did not converge. DFT calculations converged for 4445 structures that formed the calculated group, while the unconverged and large structures comprised 319 uncalculated structures. The acceptance or rejection criteria described in Section 2.4 were then applied to the CSD, calculated, and uncalculated structures. Atom typing was then applied to all of the accepted structures. A total of 8607 different atom types were identified. Various forcefield precursors were computed and reported in the ESIThis work is a large-scale computation of atom types and non-bonded parameters for MOFs. 2.2.163 exchange–correlation functional and the VASP64,65 software. Frozen-core all-electron calculations were performed using the projector augmented wave66,67 (PAW) method that uses a scalar-relativistic treatment of relaxed valence electrons and high-level relativistic treatment of frozen-core electrons.68 The PAW potentials recommended on the VASP website were used for all these calculations. The planewave energy cutoff was 400 eV. Following prior recommendation,69 the number of k-points along each lattice vector times the lattice vector length was ≥16 Å. If the k-points mesh was 1 × 1 × 1 then the Gamma point was used, otherwise we used Monkhorst–Pack70k-point grids. Real-space grids were chosen to avoid aliasing errors .69 The magnetic alignment of unpaired electron spins was optimized starting from the VASP default guess .The periodic quantum chemistry calculations of MOFs were performed using the PBE72,73 functional and def2QZVPPDD74,75 basis set. Geometries of these molecules were optimized at this level of theory.Calculations for the small organic molecules in Section 3.3 were performed using Gaussian16  with the2.2r3〉 and 〈r4〉 radial moments, and atomic spin moment were computed in the Chargemol program using DDEC6 partitioning.69,76,77rA values for which 10−4 ≤ ρavgA(rA) ≤ 10−2 e bohr−3. rA is the distance from position r⃑ to atom A's nuclear position. The fitted intercept a, slope b, and squared correlation coefficient R2 are reported. The R2 values were nearly always > 0.99 indicating nearly perfect linearity. These electron cloud parameters have several uses in molecular mechanics force fields. First, they are useful to describe charge penetration .76 Second, they are useful to describe short-range exchange-repulsion.44 van Vleet et al. showed the Born-Mayer exponential term describing short-range exchange-repulsion has an effective exponent of ∼0.84 × b.44 Although their results were derived for iterated stockholder atom78 (ISA) partitioning,44 we expect the same relation to hold for DDEC6 partitioning. Third, these electron cloud parameters are useful to parameterize dispersion damping functions  that keep the dispersion energy finite as the distance between two atoms approaches zero.44,45The electron cloud parameters fit the electron density tail of each atom in the material to an exponential decay function. Specifically, the logarithm of the spherically averaged electron density assigned to atom A was fit to a straight line74 and software , C8 (dipole–quadrupole), C9 (dipole–dipole–dipole), C10 (dipole–octupole and quadrupole–quadrupole).74,82,83 The C9 coefficients were not printed to the forcefield precursors file, because they can be readily computed74 from the printed forcefield polarizability and QDO parameters. The MCLF method includes convenient mixing rules (based on a QDO model) to easily calculate each of these dispersion coefficients between unlike atoms using only parameters of the individual atoms.74The polarizabilities, dispersion coefficients, and quantum Drude oscillator (QDO) parameters were computed using the MCLF methodsoftware . The MCL6 dispersion coefficient does not equal the r−6 coefficient of the Lennard-Jones force field.84 Because the Lennard-Jones force field does not explicitly include higher-order dispersion  terms, the Lennard-Jones r−6 coefficient must be made artificially higher than C6 to effectively compensate for the neglected C8 and C10 dispersion terms.74,84 Near the minimum energy separation between two atoms, higher-order dispersion  can contribute ∼35% of the total dispersion energy.79Of key importance, the C85,86 Three QDO parameters were computed for each atom in the material: (a) the pseudoelectron's effective charge, (b) the effective QDO frequency, and (c) the QDO's reduced mass.74,85 Force fields based on QDO models describe multibody dispersion and multibody polarization beyond the dipole approximation but require advanced simulation techniques.85–87A QDO is a quantum harmonic oscillator containing a pseudoelectron attracted to a pseudonucleus.2.3e.g., DFT) electrostatic potential over a chosen set of grid points:88Ngrid_points is the number of grid points used to compute RMSE. Vmodeloffset is the average difference between VQM(r⃑) and Vmodel(r⃑) over these grid points.89 These grid points are normally chosen to be outside the material's van der Waals surface.90 For a MOF crystal, these grid points occur inside the MOF's pores.The root mean squared error (RMSE) of an electrostatic model quantifies its error compared to the quantum mechanically computed (ρ(r⃑), was ≤10−4 e bohr−3, (ii) the grid point was no closer than 5 bohr to any atom in the material, and (iii) the grid point was closer than 12 bohr to at least one atom in the material. If any one of these three criteria were not met, the grid point was not used.In this study, the RMSE grid points were uniformly distributed in the volume of space that simultaneously met all three of the following criteria: (i) the material's total electron density, null_model(r⃑) = 0.91 Note that Vnull_modeloffset equals the average of VQM(r⃑) over the RMSE grid points, VQMavg. Therefore,76,88,91,92 co-authored by one of us and differs from the even earlier literature89,93 by including the potential offsets in this RRMSE definition. These potential offsets must be included in the RMSE and RRMSE definitions, because in periodic materials the electrostatic potential has no obvious spatial position where it approaches zero value and the energy of a system having no net charge is invariant to a constant electrostatic potential shift.The relative root mean squared error (RRMSE) is the ratio of the electrostatic model's RMSE to the RMSE of a null model for which VQM(r⃑) was output from VASP using the keyword LVHAR = .true. We wrote an OpenMP parallelized Fortran program to compute RMSE and RRMSE. The RMSE and RRMSE were computed for the following four electrostatic models: (A) NACs only (aka monopole order), (B) NACs plus spherical cloud penetration, (C) NACs plus atomic dipoles (aka dipole order), and (D) NACs plus atomic dipoles plus spherical cloud penetration.In this work, the DFT electrostatic potential V2.47 These goals were partially but not fully achieved.The 2014 CoRE MOF database was developed with goals of fixing disordered atoms, adding missing hydrogens, removing solvent molecules, discarding unfixable structures, and other cleaning protocols.To partially address remaining structural deficiencies in the 2014 CoRE MOF database, we performed: (i) reasonability checks on our computed forcefield precursors for the calculated structures and (ii) connectivity checks for all structure categories. 69,94e.g., ClO4−, BrO4−, IO4−) which can give relatively large SBOs. Oxygen atom has two electrons to share in covalent bonding but can also bond via lone-pairs ; therefore, its accepted SBO range was set to . Boron and nitrogen atoms can exhibit variable bonding involving ∼3 or ∼4 covalent bonds ; therefore, accepted SBO ranges were set to  for B and  for N. The upper bound for N was slightly higher than for B to accommodate the formally higher SBO of N in nitrates than B in borates. Since Si prefers ∼4 bonds, its accepted SBO range was set to . The accepted SBO ranges for S, Se, and Te were set to  to accommodate their ability to form ∼2  to ∼6 heuristic bonds . The accepted SBO ranges for P and As were set to  to accommodate their ability to form ∼3  to ∼6 heuristic bonds . We do not claim these choices are perfect, but they can screen out some bad structures.The sum of bond orders (SBO) was used as a screening criterion for reasonableness. DDEC6 bond orders and SBO for each atom in a material were computed using the Chargemol program.e.g., N, O, etc.).A calculated structure was rejected if any metal atom had negative NAC. In this article, the definition of metal atom included all elements not listed in A calculated structure was rejected if any one of the four RRMSE described in Section 2.3 was greater than 0.5. This criterion ensured each of our four electrostatic models described the electrostatic potential with an error less than half of a no charges model. In other words, each electrostatic model described the majority of electrostatic potential variations in the MOF's pores.Structures were rejected from all categories if they contained any isolated atoms. An atom was considered isolated if it was not connected to any other atom based on the radii listed in For CSD and uncalculated structures, some structures were rejected based on strange connectivity identified by visual inspection. Because this visual inspection was not performed systematically, we do not claim all instances of bad connectivity were identified.7 We do not report forcefield precursors for the CSD structures, because CSD licensing terms may not allow us to publicly distribute their geometries.The second column of 3.3.16, C8 and C10 dispersion coefficients; fluctuating polarizability; forcefield polarizability; electron cloud parameters; 〈r3〉 and 〈 r4〉 moments; QDO parameters; atomic dipole and quadrupole; atomic screened static polarizability tensor and isotropic polarizability; atomic spin moment. The data collected for the MOF's unit cell includes: the lattice vectors, the total spin magnetic moment, the net charge, and the RRMSE of the electrostatic potential for electrostatic models including (A) NACs only, (B) NACs plus spherical cloud penetration, (C) NACs plus atomic dipoles, and (D) NACs plus atomic dipoles and spherical cloud penetration. For each MOF, these data were written to a xyz file whose chemical structure can be visualized with the Jmol95,96 program. In the future, these forcefield precursors could be used as building blocks to construct force fields for these materials.Files containing forcefield precursors for 3056 accepted calculated structures are contained in the ESI.3.297–99 Therefore, including spherical cloud penetration (aka ‘charge penetration’) will likely improve the adsorbate–MOF and adsorbate–adsorbate electrostatic interaction energies even though its effects on RRMSE were negligible.Some additional comments are in order. Even though spherical cloud penetration had negligible effect on the RRMSE values, this does not necessarily mean charge penetration effects are not important for constructing accurate electrostatic models. In MOF's, the RRMSE probes volume in space that is likely occupied by an adsorbate atom's nuclear position. Because charge penetration extends over the volume occupied by an adsorbate atom's full electron density distribution, it affects the electrostatic potential over a much larger volume than that probed by RRMSE calculation. For this reason, charge penetration can be more important than indicated by the RRMSE values. Prior studies demonstrated intermolecular electrostatic interaction energies are substantially improved by including charge penetration.When constructing force fields, decisions have to be made about tradeoffs between simplicity and accuracy. For best accuracy, the force field should include NACs, atomic dipoles (and possibly atomic quadrupoles), and spherical charge penetration. However, the simplest force field would include NACs only and neglect atomic multipoles and charge penetration.3.329 The main idea of atom typing is to classify similar atoms into the same atom type to facilitate forcefield parameterization, where all atoms of the same atom type are normally assigned identical forcefield parameters.32 Biomolecular force fields have used atom types for several decades.100–106 The universal force field (UFF) and its extensions to MOFs  focused on atom types for structural optimizations.107–109Atom types are widely used in force fields.e.g., MOFs and covalent organic frameworks) using first neighbors only.110,111 Two significant limitations of the CBAC method are: (i) its atom types are based on first neighbors only which limits chemical transferability and (ii) the NACs for its atom types were obtained by CHELPG analysis of small fragment clusters but it is unclear how accurately these may reproduce the fully periodic electrostatic potential.110,111The connectivity based atom contribution (CBAC) method defined atom types in porous materials . Second, we reduced some transition metal radii to eliminate unreasonable metal–metal bonds and excessively high coordination numbers. Third, the carbon and oxygen radii were slightly increased to maintain carbon/oxygen–metal bonds after decreasing the metal radii. These radii values are unique only in an approximate sense, because small increases or decreases in the radii values may be feasible. Large changes in these radii values are not feasible, because bad atom connectivity would result.During atom typing, two atoms were considered directly connected if the distance between them was no greater than the sum of the atom typing radii listed in These atom type definitions gave a total of 1313 first-neighbor atom types and 7033 second-neighbor atom types for the 3056 accepted calculated MOFs. Of these, 783 first-neighbor and 3015 second-neighbor atom types appeared in more than one MOF.6, C8, and C10 dispersion coefficients; fluctuating, forcefield, and static polarizabilities; 〈r3〉 and 〈r4〉 radial moments; a, b, and R2 electron cloud parameters; atomic dipole moment magnitude; three QDO parameters; and atomic spin moment. 6 across first-neighbor-based and second-neighbor-based atom types. Only atom types appearing in more than one accepted calculated structure were included in this analysis. Second-neighbor-based atom types showed remarkably better chemical transferability compared to first-neighbor-based atom types. For example, 91.9% of the second-neighbor-based atom types had NAC standard deviations ≤0.05e, while only 59.5% of the first-neighbor-based atom types did.Is second-neighbor-based atom typing optimal? To explore this question, the averages and standard deviations of 17 different forcefield precursors were computed and listed in the ESI112 The inductive effect usually decreases across each bond and is usually limited to 2 to 3 bonds lengths.112 Our decision to base atom typing on first and second neighbors is a pragmatic one. As shown in This atom typing is theoretically justified, because in organic molecules electronic effects play a major role in group reactivity and induction contributes a significant portion of that effect. In organic chemistry, the inductive effect is the electron donating or withdrawing ability of a chemical group that can be transmitted to other parts of the molecule through chemical bonds.Do a relatively small number of atom types completely describe a large percentage of the accepted calculated structures? 7 Among the 3056 accepted calculated structures, 785 structures were built entirely of the elements Cu, Zn, C, H, N, and O. These 785 structures contained 1314 different atom types.Zn and Cu were the most common metal elements in the 2014 CoRE MOF database.et al.,62 we obtained 32 530 atom types from 130 265 molecules in the dataset (aka ‘130k’ dataset).  The DDEC6 NACs for these molecules are obtained from Bleiziffer et al.'s data for a dielectric constant of 4.62 Of the atom types from the 130k molecules and 3056 accepted calculated CoRE MOFs, 798 are shared in both datasets and 780 of these have more than one occurrence (in the same or multiple structures) in each dataset. et al. trained a machine learning model on the 130k dataset to predict DDEC6 NACs with high accuracy.62 The similar DDEC6 NAC between CoRE MOF and 130k molecules datasets for a shared atom type and Bleiziffer et al.'s successful machine learning model indicate it should be feasible to train a machine learning model to predict the properties of new atom types. Due to the extremely large number of distinct atom types we found in these datasets, a machine learning model could be highly useful to assign force-field parameter values for such a large number of atom types.Finally, we tested the transferability of atom typing across different classes of materials. Applying the second-neighbor atom typing procedure discussed above to the molecular test set of Bleiziffer 4.In this article, we considered the problem of how to automatically extract forcefield precursors from quantum chemistry calculations using DDEC6 atomic population analysis. We focused on calculating non-bonded parameters for each atom in the material: net atomic charge, atomic dipole and quadrupole, electron cloud parameters, atomic spin moment, dispersion coefficients, various polarizabilities, and QDO parameters. Our first main result was calculated values of these atomistic descriptors for 3056 MOFs that will serve as building blocks to construct classical force fields for these materials.Regarding the electrostatic parameters, our results confirm the general belief that NACs can often reproduce the electrostatic potential surrounding a material with acceptable accuracy. Including atomic dipoles dramatically reduced the electrostatic potential errors; therefore, it is preferable to include atomic dipoles in the electrostatic model. Spherical cloud penetration had negligible effect on the RRMSE histograms; however, charge penetration effects can still be important at short interatomic distances.Our second main result was the practical assessment of atom typing for MOFs. We improved values of the atom typing radii that define whether two atoms in a material are directly bonded to each other. Our results showed that atom types based on both first and second neighbors adequately captures the chemical environment, but atom types based on only first neighbors does not. Specifically, the standard deviation of calculated forcefield precursors was relatively large across atoms sharing similar first neighbor environments but relatively small across atoms sharing similar first and second neighbor environments. Including third neighbors in the atom type definition would create an unnecessarily large and burdensome number of different atom types. Therefore, atom typing including both first and second neighbors is optimal.18,19 To date, only a tiny fraction of these hypothetical MOFs have been chemically synthesized.18,19 As more and more of these hypothetical MOFs are synthesized, many atom types will be reused leading to a higher MOF to atom type ratio. Moreover, parameterizing only the popular atom types could describe a substantial percentage of MOFs with higher MOF to atom type ratio.Our results demonstrate the large chemical diversity of MOFs. 8607 different atom types were identified in the 3608 non-rejected MOFs. These atom types should be useful to develop future force fields for MOFs. Although the MOF to atom type ratio was lower than 1.0 in our study, there are two key reasons to be believe this ratio will improve in the future: (1) the number of chemical elements from which MOFs can be synthesized is practically limited to ∼100, because heavier chemical elements undergo rapid radioactive decay. Therefore, new MOFs will reuse many of the same chemical elements. (2) There is an almost infinite number of different ways to combine common metals and common organic linkers to form MOFs.e.g., DFT + dispersion) and classical force fields. The former needs orders of magnitude improvement in computational speed to yield rapid ab initio molecular dynamics. The latter requires extensive parameterization to yield accurate force fields. To actually develop working force fields, the non-bonded interaction terms studied herein will need to be combined with bonded interaction terms  and further parameterization of short-range exchange-repulsion. However, in simulations using a rigid framework approximation , the bonded interaction terms are not required.In summary, more research is urgently needed to develop accurate interaction models for MOFs. Because of the large chemical diversity of real and hypothetical MOFs, it is impractical to evaluate all possible MOFs experimentally. Therefore, computational assessment is required. The interaction model is a crucial ingredient of computational assessment. Two major types of interaction models are exchange–correlation theories  CAREER Award DMR-1555376 provided financial support. Supercomputing resources were provided by the Extreme Science and Engineering Discovery Environment (XSEDE).T. C. performed the calculations and wrote Python scripts to prepare input files, analyze output files, perform atom typing, determine whether to accept or reject structures, and write files containing force-field precursors and atom type statistics. T. A. M. wrote the programs to compute the electrostatic potential RRMSE and electron cloud parameters. T. A. M. obtained funding for the project. Both authors designed the study, interpreted data, and wrote the manuscript.There are no conflicts of interest to 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